期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 100, 页码 15975-15978出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc06519k
关键词
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资金
- Swiss National Science Foundation [200020-144471]
- EPSRC [EP/K001507/1, EP/J014753/1, EP/H035818/1]
- EC FP7 ITN MOLESCO''
- Engineering and Physical Sciences Research Council [EP/K001507/1, EP/H035818/1, EP/J014753/1] Funding Source: researchfish
- EPSRC [EP/J014753/1, EP/K001507/1, EP/H035818/1] Funding Source: UKRI
We report an electrochemical gating approach with similar to 100% efficiency to tune the conductance of single-molecule 4,40' bipyridine junctions using scanning-tunnelling-microscopy break junction technique. Density functional theory calculation suggests that electrochemical gating aligns molecular frontier orbitals relative to the electrode Fermi level, switching the molecule from an off resonance state to partial'' resonance.
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