期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 69, 页码 9872-9875出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc03493g
关键词
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资金
- Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan [24350029, 2107, 24108732, 2406, 24107004, 24850014, 25810042]
- Kyushu University Interdisciplinary Programs in Education and Projects in Research Development
- International Institute for Carbon Neutral Energy Research [WPI-I2CNER]
- World Premier International Research Center Initiative (WPI), MEXT, Japan
- Grants-in-Aid for Scientific Research [25810042, 24850014, 24108732, 24107004] Funding Source: KAKEN
A macrocyclic N-heterocyclic carbene (NHC)-cobalt complex was found to act as an improved H-2-evolving catalyst in a [Ru(bpy)(3)](2+)-sensitized photosystem using methylviologen as a redox acceptor (MV2+ + e(-) -> MV+center dot, MV2+ = N,N'-dimethyl-4,4'-bipyridinium), which provides a driving force of only 150 meV for H-2 evolution at pH 5.0.
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