期刊
CHEMICAL COMMUNICATIONS
卷 49, 期 71, 页码 7776-7778出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc44354j
关键词
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资金
- Ministry of Education, Culture, Sports, Science and Technology (Japan)
- Workshop on Chirality in Chiba University (WCCU)
- Grants-in-Aid for Scientific Research [25620075] Funding Source: KAKEN
A series of bis(oxazolidine)pyridine ligands (the PyBodines) were newly designed and synthesized for the development of a highly efficient, tailor-made catalyst for the [3+2] cycloaddition of azomethine imines with propiolates. The PyBodine(L-Ala)-Cu(OAc)(2) catalyst was selected on the basis of solid-phase catalysis/CD-HTS and exhibited high efficiency, producing the (R)-adducts with excellent enantioselectivity.
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