期刊
CHEMICAL COMMUNICATIONS
卷 48, 期 74, 页码 9266-9268出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc34577c
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资金
- MINECO of Spain [CTQ2011-29054-C02-01/BQU]
- DGR of the Generalitat de Catalunya [2009SGR462, XRQTC]
Kinetic and DFT studies revealed that protonation of Ti-containing polyoxometalates (Ti-POM) lowers significantly the energy barrier for the heterolytic oxygen transfer from the Ti hydroperoxo intermediate to the alkene, increasing the activity and selectivity of alkene oxidation.
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