期刊
CHEMICAL COMMUNICATIONS
卷 46, 期 5, 页码 704-706出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b921066k
关键词
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资金
- DOE, BES [FG02-84-ER13289]
- NSF [CHE-0513936, PHY-06-46094]
Facile, direct acylation of dimethylamine with formaldehyde to N,N-dimethylformamide proceeds with a selectivity approaching 100% at low oxygen concentrations on metallic silver surfaces; the reaction proceeds via nucleophilic attack of adsorbed dimethylamide on formaldehyde with subsequent beta-H elimination from the adsorbed hemiaminal.
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