Article
Environmental Sciences
Zijiao Yuan, Binbin He, Xiaoguo Wu, Staci L. Massey Simonich, Houqi Liu, Jiahui Fu, Afeng Chen, Hanyang Liu, Qing Wang
Summary: PAHs were the main pollutants in sediment samples from Suzhou Industrial Park, likely originating primarily from coal/biomass combustion, rather than residential and commercial activities. While most regions showed low toxicity risk levels for PAHs, vigilance is required at sampling sites with extremely high concentrations or high mean effects range?median quotient.
ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY
(2021)
Article
Environmental Sciences
Xiaoyan Ding, Xin Song, Minmin Xu, Jin Yao, Chang Xu, Zhiwen Tang, Zhuanxia Zhang
Summary: This study explores the co-occurrence and correlations of per- and polyfluoroalkyl substances (PFASs) and chlorinated volatile organic compounds (cVOCs) in field settings, finding the wide applications of substitutes for PFASs and the influence of dense non-aqueous-phase organic liquids (DNAPL) on the distribution and migration of PFASs.
SCIENCE OF THE TOTAL ENVIRONMENT
(2022)
Article
Engineering, Environmental
Ki Yong Kim, Mlamuli Ndabambi, Sol Choi, Jeong-Eun Oh
Summary: The study determined the concentrations of 28 novel and legacy PFASs in wastewater from 77 industrial plants in Korea's largest industrial complex. Only 19 and nine target PFASs were detected in untreated industrial wastewater and river water, respectively. Efforts to reduce the use of Perfluorooctane sulfonate (PFOS) have resulted in its replacement by PFASs with fewer than seven carbon atoms in both industrial wastewater and river water.
Article
Engineering, Environmental
Yibo Jia, Yumin Zhu, Dashan Xu, Xuemin Feng, Xiaoyong Yu, Guoqiang Shan, Lingyan Zhu
Summary: It has been found that some PFASs tend to accumulate in the liver and cause hepatotoxicity. Experimental results indicate that there is a competition between liver and blood for the partitioning of PFSAs, which is mainly determined by the competitive binding between hL-FABP and HSA. Therefore, the liver concentrations of PFASs in humans can be predicted from the available serum concentrations, which is important for assessing hepatotoxicity.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2022)
Article
Environmental Sciences
Chao Yin, Chang-Gui Pan, Shao-Ke Xiao, Qi Wu, Hong-Ming Tan, Kefu Yu
Summary: This study investigated the sorption, sorption isotherms, and desorption behaviors of legacy and emerging PFASs onto marine sediments at different salinities. The results showed that the adsorption of PFASs onto sediment was influenced by compound and solution-specific parameters, and salinity had a significant impact on the fate of PFASs in aquatic environments.
ENVIRONMENTAL POLLUTION
(2022)
Article
Multidisciplinary Sciences
E. R. Thomas, D. R. Tetzner, S. L. Roberts, S. D. Turner, N. L. Rose
Summary: This study provides the first evidence of the deposition of spheroidal carbonaceous particles (SCPs), which are indelible markers of industrialization, in Antarctic ice thousands of kilometers away from potential sources. The earliest observed particle was deposited in an ice layer from 1936 CE. Although deposition fluxes are low, individual SCPs were found to have originated from coal combustion based on chemical analysis.
SCIENTIFIC REPORTS
(2023)
Article
Engineering, Environmental
Pere Colomer-Vidal, Longfei Jiang, Weiping Mei, Chunling Luo, Silvia Lacorte, Anna Rigol, Gan Zhang
Summary: This study reveals that long-chain PFASs accumulate in sediment while short-chain PFASs remain in water. Floating plants absorb high levels of PFASs, while rooted species translocate short-chain PFASs from roots to shoots.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Engineering, Environmental
Yitong Pan, Damian E. Helbling
Summary: This study systematically evaluated the recovery of different lengths of PFAAs using the AOF and EOF methods and found that the EOF method is more suitable for measuring TOF in samples containing ultrashort- and short-chain PFAAs. Decreases in recovery were observed mainly due to losses during the washing step for both methods and incomplete mineralization of perfluoroalkyl sulfonic acids during combustion for the AOF method, as well as incomplete elution of short- and long-chain PFAAs and loss of ultrashort-chain PFAAs during the washing step for the EOF method.
Article
Environmental Sciences
Jose Lourenco Friedmann Angeli, Julie Rosemberg Sartoretto, Bianca Sung Mi Kim, Paulo Alves de Lima Ferreira, Beatriz Benedetti, Michel Michaelovitch de Mahiques, Rubens Cesar Lopes Figueira
Summary: The present study found historical anthropogenic mercury accumulation in the Santos estuary, with large spatial and temporal variations in mercury distribution. The highest contamination was observed in the upper estuary, with industrial activities being the primary source of mercury pollution.
MARINE POLLUTION BULLETIN
(2022)
Article
Engineering, Environmental
Guoqiang Shan, Xiang Qian, Xin Chen, Xuemin Feng, Minghong Cai, Liping Yang, Meng Chen, Lingyan Zhu, Shufeng Zhang
Summary: The distribution of PFASs in the open oceans is influenced by land-based emissions and historical residues, with PFOA mainly derived from land sources and PFOS mainly from historical residues. The new emerging compound 6:2 Cl-PFESA was found in higher concentrations near Australia. Different regions showed different sources of PFASs, with the Southern Ocean primarily influenced by atmospheric input and the Northwest Pacific Ocean and Eastern Indian Ocean mainly originating from land sources.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Environmental Sciences
Fengwen Wang, Weiru Wang, Daiyin Zhao, Jiaxin Liu, Peili Lu, Neil L. Rose, Gan Zhang
Summary: This study collected rainwater samples from Chongqing, China, over four seasons and analyzed them for 17 PFASs. The results showed that paper packaging production and AFFF usage were the major sources of PFASs, with distinct seasonal variations and wet deposition being the main pathway. This study provides important information for understanding PFASs occurrence and atmospheric wet deposition in Chongqing and other urban centers in China.
ATMOSPHERIC ENVIRONMENT
(2022)
Article
Biochemistry & Molecular Biology
Anan Ibrahim, Eric Capo, Martin Wessels, Isabel Martin, Axel Meyer, David Schleheck, Laura S. Epp
Summary: This study used historical environmental DNA data to reveal key community change points during lake eutrophication and re-oligotrophication. The research found significant shifts in the lake's community structure in recent decades, and suggested that each microbial group exhibited a unique response to environmental changes.
Article
Environmental Sciences
Celine Begorre, Aymeric Dabrin, Amandine Morereau, Hugo Lepage, Brice Mourier, Matthieu Masson, Frederique Eyrolle, Marina Coquery
Summary: This study investigated the use of the non-reactive fraction of metals in fingerprinting to estimate historical contributions of suspended particulate matter (SPM) in sediment cores. Results showed that the nonreactive fraction retained more metals in deeper layers, and tributary contributions computed using this fraction were more consistent with historical data and had lower uncertainties. This approach enables robust identification of sub-catchment areas providing large quantities of SPM.
JOURNAL OF ENVIRONMENTAL MANAGEMENT
(2021)
Article
Environmental Sciences
Xiaohua Ma, Hongbin Wan, Zhilong Zhao, Yi Li, Shuaidong Li, Changchun Huang, Tao Huang, Zhigang Zhang, Hao Yang
Summary: This study analyzed the influencing factors and sources of historical changes in polycyclic aromatic hydrocarbons (PAHs) in the sediment core of Fuxian Lake. Different sources and factors have varying impacts on PAHs before 1970, during 1971-2004, and 2005-2017.
ENVIRONMENTAL POLLUTION
(2021)
Article
Engineering, Environmental
Alexandria L. B. Forster, Ying Zhang, Danielle C. Westerman, Susan D. Richardson
Summary: Per- and polyfluoroalkyl substances (PFAS) are persistent environmental contaminants found in humans and wildlife. A new method using activated carbon adsorption, solid phase extraction, and combustion ion chromatography (CIC) was developed to measure total organic fluorine (TOF) in various environmental samples. This method provided more comprehensive measurement of PFAS compared to liquid chromatography-mass spectrometry (LC-MS), capturing known and unknown organic fluorine.
Article
Environmental Sciences
Meng Zhang, Pei Wang, Yonglong Lu, Xiaotian Lu, Anqi Zhang, Zhaoyang Liu, Yueqing Zhang, Kifayatullah Khan, Suriyanarayanan Sarvajayakesavalu
ENVIRONMENT INTERNATIONAL
(2020)
Article
Environmental Sciences
Pei Wang, Yonglong Lu, Hongqiao Su, Chao Su, Andrew C. Johnson, Longfei Yu, Alan Jenkins
ENVIRONMENT INTERNATIONAL
(2020)
Article
Environmental Sciences
Pei Wang, Meng Zhang, Qifeng Li, Yonglong Lu
Summary: The fluorochemical industry is a significant source of atmospheric PFAAs, with PFOA being dominant in the air. Inhalation of PFOA from indoor air poses a potential health risk to individuals.
ENVIRONMENT INTERNATIONAL
(2021)
Article
Engineering, Environmental
Bingnan Ren, Jing Geng, Yu Wang, Pei Wang
Summary: The study investigated the impact of tourists on PPCPs levels in wastewater in Sanya City, China, finding that tourist migrant population might be a dominant contributor. Additionally, high chronic ecological risk was identified in rivers due to the presence of dominant PPCPs.
ENVIRONMENTAL GEOCHEMISTRY AND HEALTH
(2021)
Article
Engineering, Environmental
Di Du, Yonglong Lu, Yunqiao Zhou, Qifeng Li, Meng Zhang, Guoxiang Han, Haotian Cui, Erik Jeppesen
Summary: Knowledge on bioaccumulation and trophic transfer in food webs is crucial in evaluating contaminant hazards. This study investigated the presence of PFAAs in organisms sampled from Qinzhou Bay in the South China Sea, and found different distribution patterns between short-chain and long-chain PFAAs based on trophic positions. Results suggest a potential biomagnification effect of PFOS, while the effects of PFOA were less clear. Banned long-chain PFAAs were found to still persist in the coastal marine ecosystem, while emerging short-chain PFAAs showed high concentrations but no biomagnification.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Environmental Sciences
Lu Yang, Tieyu Wang, Yunqiao Zhou, Bin Shi, Ran Bi, Jing Meng
Summary: The study revealed the presence of 30 different PPCPs in the Baiyangdian basin, with domestic sewage being the primary source and showing relatively high ecological risks, especially near the outlets of wastewater treatment plants. Effective management strategies will be needed to address this issue.
SCIENCE OF THE TOTAL ENVIRONMENT
(2021)
Article
Environmental Sciences
Bin Shi, Tieyu Wang, Hongfa Yang, Yunqiao Zhou, Ran Bi, Lu Yang, Seo Joon Yoon, Taewoo Kim, Jong Seong Khim
Summary: Polyfluoroalkyl substances (PFASs) are recognized as emerging contaminants that have captured worldwide attention due to their persistent and bioaccumulative characteristics. This study detected 15 PFASs in major rivers of rapidly developing coastal areas of China and South Korea, showing significant variations in concentrations and compositions among different regions. Time-trend analysis revealed a decrease in total PFASs concentrations in both China and South Korea, while the proportion of short-chain PFASs increased.
SCIENCE OF THE TOTAL ENVIRONMENT
(2021)
Editorial Material
Environmental Sciences
Jong Seong Khim, Tieyu Wang, Xiaowei Zhang, Seongjin Hong
ENVIRONMENT INTERNATIONAL
(2021)
Article
Green & Sustainable Science & Technology
Guangcai Yin, Hanghai Zhu, Zhiliang Chen, Chuanghong Su, Zechen He, Xinglin Chen, Jinrong Qiu, Tieyu Wang
Summary: In this study, the contents of ten heavy metals in surface soil samples from the Pearl River Delta region were investigated. The results showed that the soil quality was generally good, with slightly elevated levels of certain heavy metals compared to background values. The source apportionment analysis revealed that the majority of soil heavy metals in the PRD region could be attributed to natural and industrial sources, with smaller contributions from transportation and agricultural activities.
Article
Green & Sustainable Science & Technology
Haotian Cui, Yonglong Lu, Yunqiao Zhou, Guizhen He, Qifeng Li, Changfeng Liu, Rui Wang, Di Du, Shuai Song, Yinyi Cheng
Summary: Rapid motorization has led to vehicles becoming one of the main sources of air pollution, posing a significant risk to human health. A dynamic vehicle emission model (DVEM) was developed to accurately estimate the spatiotemporal variation and driving factors of vehicle emissions, using polycyclic aromatic hydrocarbons (PAHs) as an example. The results showed that vehicle PAHs emissions peaked in 2012 and declined in the following years due to upgraded emission standards. The emissions varied among provinces in China, with higher levels in eastern coastal provinces. Motorcycles and light duty vehicles were the main contributors to PAHs emissions. Urbanization and urban road density were found to influence the vehicle emission density. Integrated management strategies should be implemented by the government to reduce the impacts of vehicle PAHs emissions.
JOURNAL OF CLEANER PRODUCTION
(2022)
Article
Green & Sustainable Science & Technology
Jing Meng, Tieyu Wang, Bin Shi, Qianqian Li, Chenxi Wang, Lingwen Dai, Guijin Su
Summary: The ubiquitous distributions of chromium in environments pose threats to human and ecosystem health. China, as the largest producer and consumer of chromium products, has complete chromium-related industries. This study illustrated the flow of chromium from Chinese industrial sectors to the environment, with emissions through waste gas, wastewater, and solid waste being the main pathways. Ferrochromium manufacturing contributed the most to total wastes, while general solid waste treatment was the primary pathway of chromium entering the soil.
JOURNAL OF CLEANER PRODUCTION
(2022)
Article
Engineering, Environmental
Qiongping Sun, Jiaer Zhang, Tieyu Wang, Yonglong Xiong, Xinyi Zhan, Hancheng Zhao, Jianwen Wang, Yueyao Fan, Ran Bi, Shuqing Wang, Seongjin Hong, Jong Seong Khim
Summary: Perfluoroalkyl substances (PFASs) in bullfrogs, a popular aquatic food in South China, were found to pose a health risk. However, cooking methods, especially steaming, can effectively reduce PFASs concentrations, while increasing the nutritive value index (NVI). Cultured bullfrogs and steaming were recommended for consumers due to lower PFASs levels and health benefits.
JOURNAL OF HAZARDOUS MATERIALS
(2023)
Article
Environmental Sciences
Xiaohan Chen, Puhui Zhao, Difeng Wang, Lin Wang, Hancheng Zhao, Xinjie Wang, Ziyu Zeng, Ping Li, Tieyu Wang, Wenhua Liu, Ran Bi
Summary: This study investigated the seasonal variations in microplastic distribution in marine sediments in multiple-used zones of Eastern Guangdong in the South China Sea. It was found that microplastic abundance was lowest in summer, significantly lower than other seasons. The most abundant microplastic size range was 50-200 μm, and transparent and fragmented microplastics were the most frequently observed composition. Microplastic abundance was negatively correlated with distance to the coast. Seaweed ecosystems impacted microplastic abundance by changing the microenvironment and/or direct contact and entrapment. The study also identified the most frequently detected compositions and recommended appropriate management of plastic waste to reduce microplastic pollution in the marine environment.
Article
Environmental Sciences
Qiongping Sun, Tieyu Wang, Xinyi Zhan, Seongjin Hong, Lanfang Lin, Peixin Tan, Yonglong Xiong, Hancheng Zhao, Zhixin Zheng, Ran Bi, Wenhua Liu, Shuqi Wang, Jong Seong Khim
Summary: In this study, PFAS and fatty acids were tested in squids from the southeast coastal regions of China. Higher concentrations of PFAS were found in squids from the subtropical zone compared to the temperate zone. Cooking methods were effective in reducing PFAS in squids, but caution should be taken to minimize PFAS exposure through juice and oil. Squids can be considered a healthy food due to the health benefits associated with fatty acids.
ENVIRONMENT INTERNATIONAL
(2023)
Article
Environmental Sciences
Bin Shi, Yongjian Jiang, Jinshui Yang, Renxin Zhao, Tieyu Wang, Guijin Su, Yanpeng Ding, Qianqian Li, Jing Meng, Ming Hu
Summary: This study explores the relationship between the presence and ecological risk of pharmaceutical and personal care products (PPCPs) and human activity on the Qinghai-Tibet Plateau. It finds that 28 out of 30 PPCPs were detected in the region, with higher concentrations in the Tibet Autonomous Region compared to Qinghai Province. The study identifies livestock breeding as a major source of PPCP emission into soil and surface water. Furthermore, it predicts that certain PPCPs can have deleterious effects on water biota.
ENVIRONMENT INTERNATIONAL
(2023)