期刊
JOURNAL OF COLLOID AND INTERFACE SCIENCE
卷 450, 期 -, 页码 45-53出版社
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcis.2015.02.061
关键词
Graphene; N-doped La2Ti2O7; Extended light absorption; Efficient charge separation; Synergistic effect
资金
- National Natural Science Foundation of China [51308183, 51179052]
- Natural Science Foundation of Jiangsu Province of China [BK20130828]
- Fundamental Research Funds for the Central Universities [2013B32214, 2014B07414]
- Qing Lan Project
Nitrogen-doped lanthanum titanate decorated on graphene sheets (GR/N-doped La2Ti2O7) used as photocatalyst was prepared by a two-step process. To synthesize GR/N-doped La2Ti2O7, La2Ti2O7 was initially developed under heat treatment in NH3 and subsequently decorated on GR by hydrothermal processing. The resulting GR/N-doped La2Ti2O7 was characterized by scanning electron microscopy, transmission electron microscopy, atomic force microscopy. X-ray diffraction. Raman spectroscopy, and X-ray photoelectron spectroscopy. Characterization results indicated that N-doped La2Ti2O7 was approximately 6-8 nm thick with single-crystalline perovskite structure and chemically attached onto GR nanosheets by the formation of Ti-N bond, Ti-C bond, and oxynitrides. The application of GR/N-doped La2Ti2O7 composites to bisphenol A decomposition exhibits high photocatalytic efficiency under irradiation compared with pure La2Ti2O7 materials. This finding was due to the synergistic effect of great adsorption, enhanced light absorption, efficient charge separation and transfer processes in the presence of GR, and reduced band gap energy because of N doping. This study provides new insights into the fabrication and practical application of high-performance photocatalysts in wastewater treatment. (C) 2015 Elsevier Inc. All rights reserved.
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