期刊
BIOPHYSICAL JOURNAL
卷 99, 期 2, 页码 344-352出版社
CELL PRESS
DOI: 10.1016/j.bpj.2010.04.039
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资金
- Netherlands Organisation for Scientific Research
- Russian Foundation for Basic Research [09-04-00605a]
- Natural Sciences and Engineering Research Council of Canada
We model the spectra and excitation dynamics in the phycobiliprotein antenna complex PE545 isolated from the unicellular photosynthetic cryptophyte algae Rhodomonas CS24. The excitonic couplings between the eight bilins are calculated using the CIS/6-31G method. The site energies are extracted from a simultaneous fit of the absorption, circular dichroism, fluorescence, and excitation anisotropy spectra together with the transient absorption kinetics using the modified Redfield approach. Quantitative fit of the data enables us to assign the eight exciton components of the spectra and build up the energy transfer picture including pathways and timescales of energy relaxation, thus allowing a visualization of excitation dynamics within the complex.
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