期刊
ATMOSPHERIC ENVIRONMENT
卷 42, 期 14, 页码 3315-3331出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.atmosenv.2007.06.040
关键词
ammonia; hydrogen sulfide; swine barns; CAFOs
Emissions of atmospheric ammonia-nitrogen (NH3-N, where NH3-N = (14/17)NH3) and hydrogen sulfide (H2S) were measured from a finishing swine confinement house at a commercial pig farm in eastern North Carolina. Continuous simultaneous NH3-N and H2S emissions were made for similar to 1-week period during four different seasons. The number of pigs contained in the house varied from similar to 850 to 900 with average weights ranging from similar to 38 to 88 kg. Average NH3-N concentrations were highest during the winter and spring sampling periods, 8.91 +/- 4.61 and 8.44 +/- 2.40 ppm, respectively, and lower during the summer and fall, 2.45 +/- 1.14 and 4.27 +/- 0.71 ppm, respectively. Measured average H2S concentrations were 673 +/- 282, 429 +/- 223, 47 +/- 18, and 304 +/- 88 ppb during winter, spring, summer, and fall, respectively. Generally, the H2S concentrations were approximately an order of magnitude less than NH3-N during winter, spring, and fall, and two orders of magnitude smaller during the summer season. The average ambient temperature ranged from 5.5 to 22.3 degrees C while the average barn temperature measured at the outlet fans ranged from 19.0 to 26.0 degrees C in the winter and summer, respectively. The average fan ventilation rates varied from 253 m(3) min(-1) during the fall sampling period to 1024 m(3) min(-1) during summer. Calculated total emission rates for both NH3-N and H2S were highest during the spring, 4519 +/- 1639 g N day(-1) and 481 +/- 142 g day(-1), respectively. Emissions were lowest during the fall season for NH3-N (904 +/- 568 g N day(-1)) and the summer season for H2S (82 +/- 49 g day(-1)). Normalized NH3-N emission rates were highest in winter and spring (33.6 +/- 21.9 and 30.6 +/- 11.1 g N day(-1) AU(-1), where 1 AU (animal unit) = 500 kg) and lowest during summer and fall (24.3 +/- 12.4 and 11.8 +/- 7.4 g N day(-1) AU(-1)). Normalized H2S emissions were highest during the winter and spring seasons (4.2 +/- 2.1 and 3.3 +/- 1.0 g day(-1) AU(-1)) and were lowest in summer and fall (1.2 +/- 0.7 and 1.7 +/- 0.5 g day(-1) AU(-1)). (c) 2007 Elsevier Ltd. All rights reserved.
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