期刊
ASIAN JOURNAL OF CHEMISTRY
卷 25, 期 15, 页码 8471-8474出版社
ASIAN JOURNAL OF CHEMISTRY
DOI: 10.14233/ajchem.2013.14792
关键词
Nanoscale zero valent iron; Nitrate; Kinetic; Reduction
资金
- National Natural Science Foundation of China [21205001]
- National 11th Five-Year Plan Major Scientific and Technological Issues of China [2009ZX07316-004]
- Anhui Provincial Natural Science Foundation [1208085MB16]
In this study, a more fine-grained spherical nanoscale zero valent iron (nZVI) with diameter of 20-50 nm was synthesized in ethanol-water mixed solvent. The structures and physical properties of nZVI were characterized by transmission electron microscope, X-ray diffractometer analyzer. Reactivity of the nZVI was affirmed by denitrification of nitrate. The removal efficiency of nitrate in the presence of nZVI was 80 % within 1 h at optimal conditions. In view of this, the nZVI is efficient to removing nitrate and offers a great potential to the removal of other contaminants in water. The kinetic estimations in terms of three kinds model (the first-order, the second-order and the Langmuir-Hinshelwood) under the conditions of different initial nitrate concentration or different nZVI dosage were compared with each other. The result was obtained that the S-model fits the denitrification very well.
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