期刊
APPLIED PHYSICS LETTERS
卷 103, 期 26, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.4860993
关键词
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资金
- Department of Energy (DOE) through the Stanford Institute for Materials Energy Science [DE-AC02-76SF00515]
- HPSynC
- DOE-BES [DE-SC0001057, DE-FG02-99ER45775, DE-AC02-06CH11357]
- DOE-NNSA [DE-NA0001974]
- NSF
- Florida International University [DE-FG02-07ER46461]
- [NSF-EAR-1055454]
- U.S. Department of Energy (DOE) [DE-FG02-07ER46461] Funding Source: U.S. Department of Energy (DOE)
Nanoscale transmission x-ray microscopy measurements have been performed to determine the effect of pressure (P) on the volume (V) change in GeO2 glass up to 38.5 GPa. The P-V data show a continuous increase upon compression, indicating that the density-driven structural transformation is a gradual process. Over the pressure range studied, a transition is observed at approximately 10-13 GPa, where the material displays distinct compression behaviors. The pressure-induced densification that involves the coordination number change has been discussed. Using this newly developed high-pressure imaging technique with tens of nanometer resolution, we have provided a direct and unequivocal way for measuring density of amorphous materials to much higher pressures with accuracy rivaling x-ray diffraction of crystalline solids. (C) 2013 AIP Publishing LLC.
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