Article
Chemistry, Multidisciplinary
Marco Hoeppner, Bahman Kheradmand-Boroujeni, Joern Vahland, Michael Franz Sawatzki, David Kneppe, Frank Ellinger, Hans Kleemann
Summary: The high-frequency and low-voltage operation of organic thin-film transistors (OTFTs) is crucial for the commercial success of flexible electronics. While significant progress has been made, technology maturity remains a key challenge, including scalability, integrability, and device reliability.
Article
Chemistry, Multidisciplinary
Ab F. Nieuwenhuis, Daniel F. Duarte Sanchez, Jin Z. Cui, Serge G. Lemay
Summary: In this study, the quasi-1D electrical current through long single conjugated polymer chains was measured using coupled ionic-electronic charge transport. It was found that fluctuations between internal conformations of the individual polymers resulted in abrupt, multilevel switches in the electrical current, consistent with theoretical simulations. Additionally, the results provided insights into the dynamics of random-coil polymers and the potential use of semiconducting polymers as electrical labels for single-molecule sensing assays.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Guocai Liu, Qingyuan Li, Wei Shi, Yanwei Liu, Kai Liu, Xueli Yang, Mingchao Shao, Ankang Guo, Xin Huang, Fan Zhang, Zhiyuan Zhao, Yunlong Guo, Yunqi Liu
Summary: This study presents the development of multisensory artificial synapse and neural networks based on electrolyte-gated vertical organic field-effect transistors (VOFETs). With a scaled down channel length and a large electric double layer capacitance, the artificial synapse exhibits significantly lower power consumption compared to biological synapses. It is capable of learning and memory functions, as well as emulating human brain's information processing and sound detection. Additionally, the artificial synapse can be applied in acidity discrimination as an artificial tongue.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Xincan Qiu, Jing Guo, Ping-An Chen, Kaixuan Chen, Yu Liu, Chao Ma, Huajie Chen, Yuanyuan Hu
Summary: This study demonstrates that high bias-stress stability can be achieved in vertical structured OFETs (VOFETs) in combination with doping techniques, which outperforms conventional planar OFETs. By optimizing device performance and doping PDVT-10 to reduce trapping effects, the bias-stress stability of VOFETs is significantly improved. The characteristic time of doped PDVT-10 VOFETs is found to be over four times larger than that of planar PDVT-10 OFETs under the same bias-stress conditions, showing promising applications of VOFETs and effective strategy for highly bias-stress stable OFETs.
Article
Physics, Applied
Najmeh Delavari, Klas Tybrandt, Magnus Berggren, Benoit Piro, Vincent Noel, Giorgio Mattana, Igor Zozoulenko
Summary: Electrolyte-gated organic field-effect transistors (EGOFETs) are a type of organic thin-film transistors suitable for sensing and biosensing in aqueous media. They operate at low voltages by forming electric double layers and currently lack a detailed quantitative model to predict device performance.
JOURNAL OF PHYSICS D-APPLIED PHYSICS
(2021)
Article
Nanoscience & Nanotechnology
Sang Young Jeong, Jung Woo Moon, Soonyong Lee, Ziang Wu, Sung Hyeon Park, Jeong Ho Cho, Han Young Woo
Summary: In this study, a quasi-solid-state ion gel-gated vertical-type OECT (v-OECT) and NOT logic gate are successfully demonstrated by combining both p-type and n-type v-OECTs for the first time. Compared to aqueous devices, an enlarged electrochemical window and improved operational stability are observed. Logic gates are successfully demonstrated using p- and n-type v-OECTs, suggesting the potential of OECT-based next-generation electronics.
ADVANCED ELECTRONIC MATERIALS
(2023)
Article
Multidisciplinary Sciences
Larissa Huetter, Adrica Kyndiah, Gabriel Gomila
Summary: This article presents the analytical physical modeling of undoped electrolyte gated organic field effect transistors (EGOFETs) in the Helmholtz approximation. A compact analytical model for the current-voltage (I-V) characteristics, including the effects of access series resistance, has been derived and validated by 2D finite element numerical calculations. The model describes all operating regimes continuously, covers small channel lengths, and only includes physical device parameters. Analytical expressions for phenomenological parameters in the ideal FET model have been proposed. The derived analytical physical model provides a simple and quantitative way to analyze the electrical characteristics of EGOFETs beyond the oversimplified ideal FET model.
ADVANCED THEORY AND SIMULATIONS
(2023)
Article
Chemistry, Physical
Xiumei Wang, Enlong Li, Yaqian Liu, Shuqiong Lan, Huihuang Yang, Yujie Yan, Liuting Shan, Zhixian Lin, Huipeng Chen, Tailiang Guo
Summary: Stretchable organic transistors, such as the stretchable vertical organic field effect transistor (s-VOFET) and stretchable vertical synaptic transistor (s-VST), demonstrate excellent electrical properties and stability under strain. Coupling triboelectric nanogenerator (TENG) with synaptic transistors opens up new possibilities for direct interactions between environmental perception data and human-machine interfacing, paving the way for self-powered neurologically integrated artificial tactile pathways in stretchable electronics.
Article
Chemistry, Multidisciplinary
Adrica Kyndiah, Marti Checa, Francesca Leonardi, Ruben Millan-Solsona, Martina Di Muzio, Shubham Tanwar, Laura Fumagalli, Marta Mas-Torrent, Gabriel Gomila
Summary: Scanning dielectric microscopy in force detection mode in liquid environment can be used for nanoscale probing of the conductivity and interfacial capacitance in electrolyte-gated organic field-effect transistors (EGOFETs). The mapping of conductivity in the semiconducting channel reveals dependency on gate voltage and variations along the channel due to space charge limited conduction, showing very small electrical heterogeneities. These insights into transduction mechanisms at organic semiconductor/electrolyte interfaces down to approximately 100 nm can lead to substantial optimization of organic electronic devices for bioelectronic applications.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Abhinav Chandresh, Christof Woell, Lars Heinke
Summary: This study demonstrates the precise deposition of nanoporous metal-organic frameworks on graphene, yielding bilayers with excellent specificity and high sensitivity. This approach can solve the low specificity issue of graphene in sensor applications.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Nanoscience & Nanotechnology
Dandan Hao, Tianqi Chen, Pu Guo, Dapeng Liu, Xin Wang, Hao Huang, Jia Huang, Fukai Shan, Zhenyu Yang
Summary: Researchers have developed artificial optoelectronic synaptic devices based on vertical organic field-effect transistors. These devices can mimic typical biological synaptic performances and operate at low voltages, achieving ultra-low power consumption.
ADVANCED COMPOSITES AND HYBRID MATERIALS
(2023)
Article
Multidisciplinary Sciences
Marcos Luginieski, Marlus Koehler, Jose P. M. Serbena, Keli F. Seidel
Summary: A charge carrier transport model is proposed to describe the operation modes of electrolyte-gated field effect transistors and organic electrochemical transistors (OECTs), including non-ideal ones. The model considers 2D or 3D percolation transport (PT) and the influence of shallow exponential trap distribution on transport. The model is able to accurately fit experimental data from electrolyte-gated organic field effect transistors and OECTs, demonstrating its versatility.
ADVANCED THEORY AND SIMULATIONS
(2023)
Article
Materials Science, Multidisciplinary
Nicolo Lago, Marco Buonomo, Sara Ruiz-Molina, Andrea Pollesel, Rafael Cintra Hensel, Francesco Sedona, Mauro Sambi, Marta Mas-Torrent, Stefano Casalini, Andrea Cester
Summary: In this study, a blend of 2,8-Difluoro-5,11-bis(triethylsilylethynyl)anthradithiophene (diFTES-ADT) and polystyrene (PS) was used as the active material for the fabrication of dual-gate EGOFETs. A digital feedback mechanism using the back-gate electrode to dynamically compensate for the transistor threshold voltage was implemented to improve the stability of EGOFETs and enable prolonged testing. This real-time threshold voltage compensation not only stabilizes the DC output current of EGOFETs but also preserves their sensing capability for low-frequency signals.
ORGANIC ELECTRONICS
(2022)
Article
Nanoscience & Nanotechnology
Qiaoming Zhang, Adrian Tamayo, Francesca Leonardi, Marta Mas-Torrent
Summary: The study demonstrates the mutual benefits between EGOFETs and surfactants, showing that EGOFETs can enhance stability by studying surfactant aggregation behavior on metal surfaces. Exposure to high concentrations of surfactant solutions also improves operational stability of EGOFETs.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Multidisciplinary Sciences
Juhee Jeon, Sola Woo, Kyoungah Cho, Sangsig Kim
Summary: This study proposes an inverter composed of reconfigurable double-gated feedback field-effect transistors (FBFETs) and investigates its logic and memory operations through computer-aided design simulations. The proposed inverter addresses the output voltage loss issue commonly found in FBFET-based inverters and achieves the same output logic voltage as the supply voltage, demonstrating promising potential for logic-in-memory applications.
SCIENTIFIC REPORTS
(2022)
Article
Engineering, Biomedical
Giuseppina Tommasini, Gwennael Dufil, Federica Fardella, Xenofon Strakosas, Eugenio Fergola, Tobias Abrahamsson, David Bliman, Roger Olsson, Magnus Berggren, Angela Tino, Eleni Stavrinidou, Claudia Tortiglione
Summary: This study demonstrates the fabrication of functional bioelectronic interfaces in living organisms by leveraging biocatalysis. The resulting electronically conducting and electrochemically active material is fully integrated within animal tissue and can be used as a biochemical marker for animal budding and regeneration.
BIOACTIVE MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Maria Seitanidou, Maria Sygletou, Kyriaki Savva, Magnus Berggren, Emmanuel Stratakis, Daniel T. Simon
Summary: Organic electronic ion pumps (OEIPs) are a promising solution for precise local delivery of biological signaling compounds. This study presents the use of solution-processed reduced graphene oxide (RGO) as high-performance driving electrodes for OEIPs, which exhibit greater charge storage capacity and improved neurotransmitter transport compared to standard PEDOT:PSS electrodes.
ADVANCED MATERIALS INTERFACES
(2022)
Article
Energy & Fuels
Dagmawi Belaineh, Robert Brooke, Negar Sani, Mehmet Girayhan Say, Karl M. O. Hakansson, Isak Engquist, Magnus Berggren, Jesper Edberg
Summary: Sustainable electrical energy storage is a crucial scientific endeavor, and this study presents a combination of cellulose, PEDOT:PSS, and carbon derivatives for high-performing supercapacitor electrodes for printed electronics. The research shows that a small amount of PEDOT:PSS is needed to achieve optimal performance.
JOURNAL OF ENERGY STORAGE
(2022)
Article
Chemistry, Physical
Hamid Ghorbani Shiraz, Zia Ullah Khan, Daniel Pere, Xianjie Liu, Yannick Coppel, Mats Fahlman, Magnus Berggren, Radoslaw Chmielowski, Myrtil L. Kahn, Mikhail Vagin, Xavier Crispin
Summary: Hydrogen technology, with its environmentally friendly and renewable properties, is considered a breakthrough for the energy industry. A recent study found that the bifunctional electrocatalyst TaS2 has high efficiency in both the hydrogen evolution reaction and the hydrogen oxidation reaction, and organic intercalation can inhibit the former. Intercalation is seen as a potential key strategy for tuning the performance of catalysts in this family.
JOURNAL OF PHYSICAL CHEMISTRY C
(2022)
Article
Chemistry, Physical
Ayesha Sultana, Md. Mehebub Alam, Eleni Pavlopoulou, Eduardo Solano, Magnus Berggren, Xavier Crispin, Dan Zhao
Summary: Internet-of-Everything (IoE) is defined as the networked connections of things, people, data, and processes. To power distributed IoE nodes in an ecofriendly manner, researchers have developed a technology to scavenge energy from the environment and self-powered devices. By utilizing electrochemically poled cellulose nanofiber (CNF) thin films processed from water dispersions, researchers have found that these films exhibit piezoelectric characteristics, making them a promising low-cost and printable ecofriendly power source for IoE nodes.
CHEMISTRY OF MATERIALS
(2023)
Article
Chemistry, Physical
Padinhare Cholakkal Harikesh, Chi-Yuan Yang, Han-Yan Wu, Silan Zhang, Mary J. Donahue, April S. Caravaca, Jun-Da Huang, Peder S. Olofsson, Magnus Berggren, Deyu Tu, Simone Fabiano
Summary: Biointegrated neuromorphic hardware offers new protocols for recording and regulating signaling in biological systems. Previous artificial neural circuits based on silicon or negative differential resistance lack biocompatibility and ion/chemical-based modulation features. This study introduces a biorealistic conductance-based organic electrochemical neuron (c-OECN) that can emulate critical biological neural features, demonstrate stochastic spiking, and enable neurotransmitter/chemical/ion-based modulation. These c-OECNs have the potential for in vivo stimulation of biological nerves.
Article
Nanoscience & Nanotechnology
Mert Vural, Mohsen Mohammadi, Laura Seufert, Shaobo Han, Xavier Crispin, Anders Fridberger, Magnus Berggren, Klas Tybrandt
Summary: Soft vibrotactile devices are important for future developments of multifunctional electronic skin technologies, but currently lack overall performance, sensing-actuation feedback, control, and mechanical compliance. This study presents soft haptic electromagnetic actuators that address these issues by utilizing intrinsically stretchable conductors, pressure-sensitive conductive foams, and soft magnetic composites.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Review
Chemistry, Multidisciplinary
Yifei Luo, Mohammad Reza Abidian, Jong-Hyun Ahn, Deji Akinwande, Anne M. Andrews, Markus Antonietti, Zhenan Bao, Magnus Berggren, Christopher A. Berkey, Christopher John Bettinger, Jun Chen, Peng Chen, Wenlong Cheng, Xu Cheng, Seon-Jin Choi, Alex Chortos, Canan Dagdeviren, Reinhold H. Dauskardt, Chong-an Di, Michael D. Dickey, Xiangfeng Duan, Antonio Facchetti, Zhiyong Fan, Yin Fang, Jianyou Feng, Xue Feng, Huajian Gao, Wei Gao, Xiwen Gong, Chuan Fei Guo, Xiaojun Guo, Martin C. Hartel, Zihan He, John S. Ho, Youfan Hu, Qiyao Huang, Yu Huang, Fengwei Huo, Muhammad M. Hussain, Ali Javey, Unyong Jeong, Chen Jiang, Xingyu Jiang, Jiheong Kang, Daniil Karnaushenko, Ali Khademhosseini, Dae-Hyeong Kim, Il-Doo Kim, Dmitry Kireev, Lingxuan Kong, Chengkuo Lee, Nae-Eung Lee, Pooi See Lee, Tae-Woo Lee, Fengyu Li, Jinxing Li, Cuiyuan Liang, Chwee Teck Lim, Yuanjing Lin, Darren J. Lipomi, Jia Liu, Kai Liu, Nan Liu, Ren Liu, Yuxin Liu, Yuxuan Liu, Zhiyuan Liu, Zhuangjian Liu, Xian Jun Loh, Nanshu Lu, Zhisheng Lv, Shlomo Magdassi, George G. Malliaras, Naoji Matsuhisa, Arokia Nathan, Simiao Niu, Jieming Pan, Changhyun Pang, Qibing Pei, Huisheng Peng, Dianpeng Qi, Huaying Ren, John A. Rogers, Aaron Rowe, Oliver G. Schmidt, Tsuyoshi Sekitani, Dae-Gyo Seo, Guozhen Shen, Xing Sheng, Qiongfeng Shi, Takao Someya, Yanlin Song, Eleni Stavrinidou, Meng Su, Xuemei Sun, Kuniharu Takei, Xiao-Ming Tao, Benjamin C. K. Tee, Aaron Voon-Yew Thean, Tran Quang Trung, Changjin Wan, Huiliang Wang, Joseph Wang, Ming Wang, Sihong Wang, Ting Wang, Zhong Lin Wang, Paul S. Weiss, Hanqi Wen, Sheng Xu, Tailin Xu, Hongping Yan, Xuzhou Yan, Hui Yang, Le Yang, Shuaijian Yang, Lan Yin, Cunjiang Yu, Guihua Yu, Jing Yu, Shu-Hong Yu, Xinge Yu, Evgeny Zamburg, Haixia Zhang, Xiangyu Zhang, Xiaosheng Zhang, Xueji Zhang, Yihui Zhang, Yu Zhang, Siyuan Zhao, Xuanhe Zhao, Yuanjin Zheng, Yu-Qing Zheng, Zijian Zheng, Tao Zhou, Bowen Zhu, Ming Zhu, Rong Zhu, Yangzhi Zhu, Yong Zhu, Guijin Zou, Xiaodong Chen
Summary: Humans are increasingly relying on flexible sensors to address challenges and improve quality of life in the digital and big data era. However, the market adoption of flexible sensors is still limited despite advancements in research. In this paper, we identify the bottlenecks hindering the maturation of flexible sensors and propose potential solutions to expedite their deployment and commercialization.
Article
Chemistry, Physical
Hamid Ghorbani Shiraz, Zia Ullah Khan, Daniel Pere, Xianjie Liu, Yannick Coppel, Mats Fahlman, Mikhail Vagin, Radoslaw Chmielowski, Myrtil L. Kahn, Magnus Berggren, Xavier Crispin
Summary: We investigated the effect of oxygen poisoning on the efficiency of hydrogen production and found that the oxygenated and intercalated electrocatalyst has a significantly lower exchange current density of the hydrogen evolution reaction compared to the pristine material.
JOURNAL OF PHYSICAL CHEMISTRY C
(2023)
Article
Chemistry, Multidisciplinary
Diana Priyadarshini, Chiara Musumeci, David Bliman, Tobias Abrahamsson, Caroline Lindholm, Mikhail Vagin, Xenofon Strakosas, Roger Olsson, Magnus Berggren, Jennifer Y. Gerasimov, Daniel T. Simon
Summary: Seamless integration between biological systems and electrical components is essential for understanding and combating neurological disorders. By employing bioelectronic systems made up of conjugated polymers, which can transport electronic and ionic charges, it is possible to achieve this integration. The enzyme-mediated polymerization of thiophene-based monomers on a synthetic lipid bilayer provides insights into their interactions with a cell membrane model, suggesting their potential for in vivo neural therapeutics.
Article
Engineering, Biomedical
Dennis Cherian, Arghyamalya Roy, Alex Bersellini Farinotti, Tobias Abrahamsson, Theresia Arbring Sjostrom, Klas Tybrandt, David Nilsson, Magnus Berggren, Camilla I. Svensson, David J. Poxson, Daniel T. Simon
Summary: The organic electronic ion pump (OEIP) is a drug delivery device that enables drug delivery without pressure or volume changes. It utilizes polyelectrolyte membranes to conduct and deliver ionic drugs with high spatiotemporal resolution. An inkjet printable formulation of polyelectrolyte is developed to simplify the fabrication process of OEIP devices, and it shows favorable iontronic characteristics. The technology is demonstrated to transport and deliver the pharmaceutical compound bupivacaine with high spatial precision and effective nerve blocking, indicating its potential for biomedical scenarios.
ADVANCED HEALTHCARE MATERIALS
(2023)
Article
Pharmacology & Pharmacy
Arghyamalya Roy, Alex Bersellini Farinotti, Theresia Arbring Sjostrom, Tobias Abrahamsson, Dennis Cherian, Michal Karaday, Klas Tybrandt, David Nilsson, Magnus Berggren, David J. Poxson, Camilla I. Svensson, Daniel T. Simon
Summary: The authors demonstrate the effective delivery of the commonly used analgesic drug bupivacaine to DRG neurons via organic electronic ion pumps (OEIPs) without fluid flow. Only cells close to the OEIP outlet are affected, at concentrations significantly lower than with bulk/bolus delivery. This achievement represents a significant milestone for the translation of this technology.
ADVANCED THERAPEUTICS
(2023)
Article
Multidisciplinary Sciences
Adam Armada-Moreira, Abdul Manan Dar, Zifang Zhao, Claudia Cea, Jennifer Gelinas, Magnus Berggren, Alex Costa, Dion Khodagholy, Eleni Stavrinidou
Summary: We developed a conformable multielectrode array based on organic electronics and used it to study the electrical signals in plants. By mapping the action potential in Venus flytrap, we discovered its propagation characteristics and its correlation with trap movement. We also found that cells other than sensory hairs can activate the Venus flytrap circuitry. This work contributes to the understanding of electrical signaling in plants and its role in long-distance responses.
Article
Chemistry, Physical
Scott T. Keene, Viktor Gueskine, Magnus Berggren, George G. Malliaras, Klas Tybrandt, Igor Zozoulenko
Summary: Efficient transport of both ionic and electronic charges in conjugated polymers has enabled a wide range of novel electrochemical devices. This Perspective provides an overview of the fundamental physical processes underlying the operation of mixed conducting polymer devices and highlights recent advances in this field. Challenges in further extending the understanding of MCP-based device operation are identified. A deeper understanding of the elementary processes governing operation in MCPs will drive materials design and device performance advancement.
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
(2022)
Correction
Chemistry, Multidisciplinary
Daniela Parker, Yohann Daguerre, Gwennael Dufil, Daniele Mantione, Eduardo Solano, Eric Cloutet, Georges Hadziioannou, Torgny Nasholm, Magnus Berggren, Eleni Pavlopoulou, Eleni Stavrinidou
MATERIALS HORIZONS
(2022)