期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 54, 期 4, 页码 1130-+出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201409714
关键词
isomers; layered compounds; metastable compounds; nanostructures; solid-state reactions
资金
- National Science Foundation [DMR-1266217]
- National Science Foundation through CCI [CHE-1102637]
- [MRI 0923577]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1102637] Funding Source: National Science Foundation
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [1266217] Funding Source: National Science Foundation
The structure of precursors is used to control the formation of six possible structural isomers that contain four structural units of PbSe and four structural units of NbSe2: [(PbSe)(1.14)](4)[NbSe2](4), [(PbSe)(1.14)](3)[NbSe2](3)[(PbSe)(1.14)](1)[NbSe2](1), [(PbSe)(1.14)](3)[NbSe2](2)[(PbSe)(1.14)](1)[NbSe2](2), [(PbSe)(1.14)](2)[NbSe2](3)[(PbSe)(1.14)](2)[NbSe2](1), [(PbSe)(1.14)](2)[NbSe2](2)[(PbSe)(1.14)](1)[NbSe2](1)[(PbSe)(1.14)](1)[NbSe2](1), [(PbSe)(1.14)](2)[NbSe2](1)[(PbSe)(1.14)](1)[NbSe2](2)[(PbSe)(1.14)](1)[NbSe2](1). The electrical properties of these compounds vary with the nanoarchitecture. For each pair of constituents, over 20000 new compounds, each with a specific nanoarchitecture, are possible with the number of structural units equal to 10 or less. This provides opportunities to systematically correlate structure with properties and hence optimize performance.
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