期刊
ADVANCED OPTICAL MATERIALS
卷 6, 期 17, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adom.201701334
关键词
2D materials; molybdenum ditelluride; phase transitions; second harmonic generation
资金
- National Natural Science Foundations of China [61522507, 61775183, 11634010]
- Key Research and Development Program [2017YFA0303800]
- Key Research and Development Program in Shaanxi Province of China [2017KJXX-12]
- Fundamental Research Funds for the Central Universities [3102017jc01001]
Optical second harmonic generations (SHGs) from atomically thin MoTe2 flakes with 2H and 1T' phases are studied. From 2H-MoTe2 samples with odd (even) numbers of layers, strong (negligible) SHGs are observed due to the layer-dependent broken inversion symmetry. When pumped by a telecom-band laser, SHG from a monolayer 2H-MoTe2 is about one order of magnitude stronger than that from a monolayer WS2; an extremely high second-order nonlinear susceptibility of 2.5 nm V-1 is estimated, presenting the highest value among those reported in 2D materials. SHG measurements in MoTe2 are also demonstrated as an efficient way to distinguish the 2H-to-1T' phase transition. Compared with the SHG in 2H-MoTe2, 1T'-MoTe2's SHG has much lower efficiency and the polarization dependence is changed from a six-fold pattern to a two-lobe pattern.
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