期刊
NANO-MICRO LETTERS
卷 10, 期 3, 页码 -出版社
SHANGHAI JIAO TONG UNIV PRESS
DOI: 10.1007/s40820-018-0196-2
关键词
Formamidinium lead trihalide (FAPbBr(3)); Perovskite microcrystals; Photodetector; External quantum efficiency
资金
- National Key R@D Program of China [2017YFA0204800]
- National Natural Science Foundation of China [21533010, 21321091, 21525315, 91333116, 21173169]
Because of the good thermal stability and superior carrier transport characteristics of formamidinium lead trihalide perovskite HC(NH2)(2)PbX3 (FAPbX(3)), it has been considered to be a better optoelectronic material than conventional CH3NH3PbX3 (MAPbX(3)). Herein, we fabricated a FAPbBr(3) microcrystal-based photodetector that exhibited a good responsivity of 4000 A W-1 and external quantum efficiency up to 10(6)% under one-photon excitation, corresponding to the detectivity greater than 10(14) Jones. The responsivity is two orders of magnitude higher than that of previously reported formamidinium perovskite photodetectors. Furthermore, the FAPbBr(3) photodetector's responsivity to two-photon absorption with an 800-nm excitation source can reach 0.07 A W-1, which is four orders of magnitude higher than that of its MAPbBr(3) counterparts. The response time of this photodetector is less than 1 ms. This study provides solid evidence that FAPbBr(3) can be an excellent candidate for highly sensitive and fast photodetectors.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据