期刊
PHYSICAL REVIEW LETTERS
卷 120, 期 12, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.120.125901
关键词
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资金
- FAPERJ fellowship (Nota 10)
- FAPERJ fellowship (Visitante)
- Fonds ESPCI
- QuantEmX Grant from ICAM [GBMF5305]
- Gordon and Betty Moore Foundation
We present a study of thermal conductivity, kappa, in undoped and doped strontium titanate in a wide temperature range (2-400 K) and detecting different regimes of heat flow. In undoped SrTiO3, kappa evolves faster than cubic with temperature below its peak and in a narrow temperature window. Such behavior, previously observed in a handful of solids, has been attributed to a Poiseuille flow of phonons, expected to arise when momentum-conserving scattering events outweigh momentum- degrading ones. The effect disappears in the presence of dopants. In SrTi1- xNbxO3, a significant reduction in lattice thermal conductivity starts below the temperature at which the average inter-dopant distance and the thermal wavelength of acoustic phonons become comparable. In the high-temperature regime, thermal diffusivity becomes proportional to the inverse of temperature, with a prefactor set by sound velocity and Planckian time (tau(p) = (h/k(B)T)).
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