期刊
PHYSICAL REVIEW LETTERS
卷 121, 期 2, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.121.023201
关键词
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资金
- Fonds de recherche du Quebec-Nature et technologies (FRQNT)
- Natural Sciences and Engineering Research Council of Canada (NSERC)
- Canada Foundation for Innovation-Major Science Initiatives
- RSF [16-12-10279]
- Russian Science Foundation [16-12-10279] Funding Source: Russian Science Foundation
High harmonics from laser-ablated plumes are mostly generated from ionic species. We demonstrate that with ultrashort infrared (similar to 1.82 mu m) driving lasers, high harmonics from laser-ablated manganese are predominantly generated from neutral atoms, a transition metal atom with an ionization potential of 7.4 eV. Our results open the possibility to advance laser-ablation technique to study the dynamics of neutral atoms of low ionization potential. Moreover, as manganese contains giant autoionizing resonance, intense and broadband high harmonics have been demonstrated from this resonance at energies from 49 to 53 eV. This opens the possibility to generate intense attosecond pulses directly from the giant resonances, as well as to study these resonances using high-harmonic spectroscopy.
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