期刊
ORGANIC LETTERS
卷 20, 期 11, 页码 3362-3366出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b01281
关键词
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资金
- Indian Institute of Technology Madras [CHY/16-17/840/RFIR/ANBA]
- CSIR, New Delhi
An efficient and chemodivergent palladium-catalyzed thiolation (C-S) and imidation (C-N) of directing group assisted C-H bonds have been accomplished employing N-(arylthio)imides in combination with either Bronsted acid or Lewis acid, respectively. Notable features of the developed methodologies include excellent diversity, high functional group tolerance, wide substrate scope, and use of a single N-S reagent. Importantly, the developed hypothesis was also successfully extended to the amidation of C-H bonds. A plausible mechanistic pathway was proposed based on the preliminary mechanistic study.
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