期刊
OPTICAL MATERIALS
卷 81, 期 -, 页码 45-54出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.optmat.2018.05.011
关键词
Exciton-plasmon coupling; Surface plasmons; 2D grating; Rhodamine-B; Rhodamine-6G; Nanoimprint lithography
The proximity of metal and semiconductor nanostructures leads to the emergence of new optical features for many tunable applications, which affects the electromagnetic modes in metallic nanostructure and electronic states in semiconductor nanostructure in nanometer scales. Thus, it will create some changes in the transition matrix elements and the absorption and emission properties. Therefore, absorption and emission properties can be designed and controlled by exciton-plasmon interaction. In the present study, Rhodamine-B and 6G were used as organic dyes in Polyvinylpyrrolidone as host medium and two-dimensional crystal as plasmonic ones. To this aim, Nano imprint lithography was used to produce two dimensional crystals and its deposit gold was utilized to harvest plasmonic mold in the proximity of excitonic media. Then, the dispersion relation was measured and the polar diagram was plotted for different coupling regime. Based on the results, this system has a poor capability for overcoming the difficulties of obtaining strong coupling although different figures of merit were observed for increasing coupling strength, which is very useful for designing and constructing new generation of plexitonic structures.
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