4.8 Article

Ultrafast saturable absorption in TiS2 induced by non-equilibrium electrons and the generation of a femtosecond mode-locked laser

期刊

NANOSCALE
卷 10, 期 20, 页码 9608-9615

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/c8nr01573b

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资金

  1. Guangdong Natural Science Foundation [S2011030001349]
  2. Natural Science Foundation of Zhejiang Province [LQ18A040004]
  3. Open Fund of the State Key Laboratory of Luminescent Materials and Devices (South China University of Technology) [2018-skllmd-13]
  4. National Natural Science Foundation of China [51302087, 51772270, 51472091]
  5. National Key R&D program of China [2018YFB1107200]

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Non-equilibrium electrons induced by ultrafast laser excitation in a correlated electron material can disturb the Fermi energy as well as optical nonlinearity. Here, non-equilibrium electrons translate a semiconductor TiS2 material into a plasma to generate broad band nonlinear optical saturable absorption with a sub-picosecond recovery time of similar to 768 fs (corresponding to modulation frequencies over 1.3 THz) and a modulation response up to similar to 145%. Based on this optical nonlinear modulator, a stable femtosecond mode-locked pulse with a pulse duration of similar to 402 fs and a pulse train with a period of similar to 175.5 ns is observed in the all-optical system. The findings indicate that non-equilibrium electrons can promote a TiS2-based saturable absorber to be an ultrafast switch for a femtosecond pulse output.

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