4.8 Article

Strongly Cavity-Enhanced Spontaneous Emission from Silicon-Vacancy Centers in Diamond

期刊

NANO LETTERS
卷 18, 期 2, 页码 1360-1365

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.7b05075

关键词

Purcell enhancement; single-photon generation; defect-center materials; diamond; silicon-vacancy center; nanophotonics; color center

资金

  1. Department of Energy (DOE), Laboratory Directed Research and Development program at SLAC National Accelerator Laboratory [DE-AC02-76SF00515]
  2. Army Research Office (ARO) [W911NF1310309]
  3. Air Force Office of Scientific Research (AFOSR) MURI Center for Quantum Metaphotonics and Metamaterials
  4. Air Force Office of Scientific Research (AFOSR) MURI Center for Attojoule Nano-Optoelectronics [FA9550-17-1-0002]
  5. National Science Foundation (NSF) [ECS-9731293, DMR-1503759]
  6. Stanford Nano Shared Facility
  7. ONR MURI on Quantum Optomechanics [N00014-15-1-2761]
  8. National Science Foundation (NSF) EFRI ACQUIRE program [5710004174]
  9. Army Research Laboratory
  10. National Science Foundation [ECS-0335765]
  11. Direct For Mathematical & Physical Scien
  12. Division Of Materials Research [1503759] Funding Source: National Science Foundation

向作者/读者索取更多资源

Quantum emitters are an integral component for a broad range of quantum technologies, including quantum communication, quantum repeaters, and linear optical quantum computation. Solid-state color centers are promising candidates for scalable quantum optics due to their long coherence time and small inhomogeneous broadening. However, once excited, color centers often decay through phonon-assisted processes, limiting the efficiency of single-photon generation and photon-mediated entanglement generation. Herein, we demonstrate strong enhancement of spontaneous emission rate of a single silicon-vacancy center in diamond embedded within a monolithic optical cavity, reaching a regime in which the excited-state lifetime is dominated by spontaneous emission into the cavity mode. We observe 10-fold lifetime reduction and 42-fold enhancement in emission intensity when the cavity is tuned into resonance with the optical transition of a single silicon-vacancy center, corresponding to 90% of the excited-state energy decay occurring through spontaneous emission into the cavity mode. We also demonstrate the largest coupling strength (g/2 pi = 4.9 +/- 0.3 GHz) and cooperativity (C = 1.4) to date for color-center-based cavity quantum electrodynamics systems, bringing the system closer to the strong coupling regime.

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