期刊
GREEN CHEMISTRY
卷 17, 期 6, 页码 3260-3265出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4gc02542c
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资金
- ZJNSF [LR14B020002]
- NNSFC [20902070]
- 580 Oversea Talents Program of Wenzhou City
Catalyst-free autocatalyzed dehydrative N-alkylation reactions of 2-aminobenzothiazoles, 2-aminopyrimidines, and 2-aminopyrazine with primary and secondary alcohols have been achieved for efficient, practical, and green synthesis of the versatile heteroaryl amine derivatives. These reactions were interestingly induced by structure-dependent tautomeric equilibria of the heteroaryl amines via MPV-O transfer hydrogenation of the imino tautomers by alcohols to give aldehydes as the key initiating step.
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