4.7 Article

Ag nanoparticles loading of polypyrrole-coated superwetting mesh for on-demand separation of oil-water mixtures and catalytic reduction of aromatic dyes

期刊

JOURNAL OF COLLOID AND INTERFACE SCIENCE
卷 527, 期 -, 页码 187-194

出版社

ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcis.2018.05.048

关键词

Polypyrrole; Ag nanoparticles; Underoil superhydrophobicity; Underwater superoleophobicity; On-demand separation; Dye degradation

资金

  1. National Nature Science Foundation of China [51522510, 51675513, 51735013]

向作者/读者索取更多资源

Herein, a catalytic mesh with unique wettability, high oil-water separation efficiency and excellent catalytic performance towards aromatic dyes was fabricated. Polypyrrole (PPy) was firstly pre-coated on pristine stainless-steel mesh (SSM) surface via cyclic voltammetry approach. Subsequently, a simple electrodeposition process was performed to prepare and anchor Ag nanoparticles (AgNPs) onto the PPycoated SSM surface. The PPy-coated mesh with anchored AgNPs was denoted as PPy/AgNPs-coated SSM. The obtained PPy/AgNPs-coated SSM exhibited dual superlyophobic properties and were able to achieve on-demand separation to deal with various of light oil (p(oil) < P-water) and heavy oil (p(oil) > P-water)water mixtures. Importantly, benefitting from AgNPs on mesh surface, the obtained PPy/AgNPs-coated SSM exhibits exceptional catalytic activity. As proof-of-concept three typical aromatic dye molecules (methylene blue, rhodamine B and Congo red) can be effectivity degraded. Additionally, the degradation of aromatic dyes and oil-water separation were achieved simultaneously when the PPy/AgNPs-coated SSM was converted to water-removing mode. Therefore, the present work is of great significance to the development of novel oil-water filtration membranes and can open a new avenue towards the practicability of metal nanoparticle catalysts in wastewater treatment. (C) 2018 Elsevier Inc. All rights reserved.

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