4.4 Article

A high-performance carbon-carbon(C/C) Quasi-Solid-State Supercapacitor with Conducting Gel Electrolyte

期刊

出版社

ESG
DOI: 10.20964/2018.03.73

关键词

Quasi-solid-state supercapacitors; PAM-G matrix; Three-dimensional structure; Energy storage

资金

  1. National Natural Science Foundation of China [21503202, 61604143, 61774139]
  2. Shandong Provincial Natural Science Foundation [ZR2015EM024]
  3. Fundamental Research Funds for the Central Universities [201564002, 201762018]

向作者/读者索取更多资源

The development of the electric double-layer capacitors (EDLCs) that pursue for the advantages of easily carrying, no leaking and high capacitance has been a strong objective at the moment. Here a new type gel electrolyte with a high special conductivity of 15.06 mS.cm(-2) was fabricate by immersing polyacrylamide gel (PAM-G) matrix in 6 M KOH aqueous solution for 60 hours. As expected, the assembled quasi-solid-state supercapacitor based PAM-G electrolyte exhibits a specific capacitance (of 196 F.g(-1) and 156 F.g(-1) at the charge-discharge current density of 1 A.g(-1) and 10 A.g(-1), respectively), maximum power of 10 kW.kg(-1) along with energy density of 28.6 Wh.kg(-1) (under the current density of 10 A.g(-1)), and the capacitance retention rate keeps 98% after 5000 cycles at 1 A.g(-1), demonstrating a high cycling stability, an excellent rate capability as well as a high specific capacitance of the device. The promising electrochemical performance could be attributed to the unique homogeneous and microporous three-dimensional structure of the PAM-G which can greatly enhance the permeability and transportation of different ions.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.4
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Environmental Sciences

Shape-controlled hollow Cu2O@CuS nanocubes with enhanced photocatalytic activities towards degradation of tetracycline

Zhenliang Li, Xuerui Liu, Shuye Li, Enke Feng, Zhiqiang Wu, Zhiming Yang, Xinxian Ma, Xinning Han

Summary: In this study, shape-controlled Cu2O@CuS nanocubes were successfully prepared and used as photocatalyst materials for the degradation of tetracycline. The experimental results showed that the nanocubes exhibited high degradation efficiency under visible light and maintained a high degradation performance even after multiple uses.

ENVIRONMENTAL TECHNOLOGY (2023)

Article Engineering, Manufacturing

Effect of isothermal storage on the microstructure and grain orientation of Cu/Cu3Sn/Cu solder joint

Gangli Yang, Xiaoyan Li, Xu Han, Shanshan Li

Summary: This study investigated the changes in microstructure and grain orientation of the Cu3Sn solder joint during isothermal aging at 420 degrees C. It was found that the original Cu3Sn solder joint transformed into full Cu(41)Sn(11) solder joint and eventually into full alpha(Cu) solder joint during aging. The formation of micro-voids during the conversion process resulted in lower reliability of the solder joint. The average grain sizes of interfacial phases exhibited an initial increase followed by a decrease during aging. The preferred orientations of the different phases were also examined.

SOLDERING & SURFACE MOUNT TECHNOLOGY (2023)

Review Biotechnology & Applied Microbiology

An updated review of SARS-CoV-2 detection methods in the context of a novel coronavirus pandemic

Yuxuan Zhang, Zhiwei Huang, Jiajie Zhu, Chaonan Li, Zhongbiao Fang, Keda Chen, Yanjun Zhang

Summary: The World Health Organization has reported over 430 million confirmed cases of COVID-19 worldwide, with nearly 6 million deaths. There is a growing need for technologies that can accurately and quickly detect the SARS-CoV-2 virus at early stages. While the qRT-PCR assay is considered the gold standard, it still has limitations. New nucleic acid detection devices and serological testing technologies are being developed, and the demand for specific detection of mutant strains is increasing due to the emergence of highly infectious variants.

BIOENGINEERING & TRANSLATIONAL MEDICINE (2023)

Article Oncology

Toripalimab Plus Chemotherapy for Patients With Treatment-Naive Advanced Non-Small-Cell Lung Cancer: A Multicenter Randomized Phase III Trial (CHOICE-01)

Zhijie Wang, Lin Wu, Baolan Li, Ying Cheng, Xiaoling Li, Xicheng Wang, Liang Han, Xiaohong Wu, Yun Fan, Yan Yu, Dongqing Lv, Jianhua Shi, Jianjin Huang, Shaozhang Zhou, Baohui Han, Guogui Sun, Qisen Guo, Youxin Ji, Xiaoli Zhu, Sheng Hu, Wei Zhang, Qiming Wang, Yuming Jia, Ziping Wang, Yong Song, Jingxun Wu, Meiqi Shi, Xingya Li, Zhigang Han, Yunpeng Liu, Zhuang Yu, An-Wen Liu, Xiuwen Wang, Caicun Zhou, Diansheng Zhong, Liyun Miao, Zhihong Zhang, Hui Zhao, Jun Yang, Dong Wang, Yingyi Wang, Qiang Li, Xiaodong Zhang, Mei Ji, Zhenzhou Yang, Jiuwei Cui, Beili Gao, Buhai Wang, Hu Liu, Lei Nie, Mei He, Shi Jin, Wei Gu, Yongqian Shu, Tong Zhou, Jian Feng, Xinmei Yang, Cheng Huang, Bo Zhu, Yu Yao, Xiongwen Tang, Jianjun Yu, Ellen Maher, Hui Feng, Sheng Yao, Patricia Keegan, Jie Wang

Summary: The CHOICE-01 study investigated the efficacy and safety of toripalimab in combination with chemotherapy as a first-line treatment for advanced non-small-cell lung cancer (NSCLC). The study found that toripalimab plus chemotherapy significantly improved progression-free survival (PFS) and overall survival (OS) compared to placebo.

JOURNAL OF CLINICAL ONCOLOGY (2023)

Article Geosciences, Multidisciplinary

Patterns and driving mechanism of soil organic carbon, nitrogen, and phosphorus stoichiometry across northern China's desert-grassland transition zone

Jiannan Lu, Shuang Feng, Shaokun Wang, Baolong Zhang, Zhiying Ning, Ruixiong Wang, Xueping Chen, Liangliang Yu, Hongsheng Zhao, Dengming Lan, Xueyong Zhao

Summary: Soil nutrient stoichiometry plays a crucial role in the ecological functioning of the desert-grassland transition zone. This study investigated the spatial pattern of soil nutrient stoichiometry and identified the key factors driving its variation. The results showed that soil nutrient contents and ratios differed among vegetation types, soil types, and soil depths. Precipitation, silt and clay content were found to be the most critical factors influencing soil nutrient stoichiometry. These findings highlight the importance of climate and soil property in shaping soil nutrient dynamics and provide insights into the impacts of future climate change on ecosystem functioning in this transition zone.

CATENA (2023)

Article Chemistry, Applied

?A-?-A? type naphthalimide-based cathode interlayers for efficient organic solar cells

Hao Liu, Shaonan Liu, Yong Zhao, Jilei Jiang, Xiaoran Feng, Mingliang Sun, Liangmin Yu, Shuixing Dai

Summary: In this work, two small molecules based on N-dimethylamino-propyl-1,8-naphthalimide with different It-bridges, ONTN and ONBN, were designed and synthesized as cathode interfacial materials (CIMs) for efficient organic solar cells (OSCs). Compared with ONBN, ONTN showed higher thermal stability, red-shift absorption, lower LUMO and higher HOMO energy levels, higher electron mobility and conductivity, and more uniform film morphology. The OSCs based on ONTN achieved a higher power conversion efficiency (PCE) of 10.38% compared to the control device of ONBN (PCE of 9.04%).

DYES AND PIGMENTS (2023)

Article Chemistry, Applied

Comprehensive application possibility: Construction hydrophilic, amphiphilic and hydrophobic system of modified zein by enzymatic or cysteine modification

An-Qi Zhang, Xiao-Yan Li, Bo-Hao Liu, Yu-Qi Yin, Han -Lin Zhang, Ying-Hua Zhang

Summary: By introducing hydrophilic groups into zein, the interaction between zein and water can be changed, which expands its application in the food industry. This study constructed hydrophilic, amphiphilic, and hydrophobic systems of zein through modification methods, and explored the structure and properties of the modified zein. Experimental results showed that the zein-potassium oleate system is hydrophobic, enzymatic modification can obtain a hydrophilic system, and cysteine modification can obtain an amphiphilic system. Various analysis methods also confirmed the hydrophilic and hydrophobic systems obtained by different modification methods. UV, IR, and fluorescence spectra of zein after enzymatic hydrolysis and cysteine modification indicated changes in the hydrophilicity and hydrophobicity of the zein microenvironment. This study provides a feasible approach to broaden the application of zein in the food industry.

FOOD HYDROCOLLOIDS (2023)

Article Green & Sustainable Science & Technology

Enhanced short chain fatty acids production from anaerobic fermentation of primary sludge using free ammonia pretreatment

Jiamin Zhang, Dongbo Wang, Xiaoming Li, Xuran Liu, Qi Yang, Qiuxiang Xu, Guojing Yang, Abing Duan, Yingchun Fang

Summary: This study introduces a new FA pretreatment technique for recovering SCFAs from PS. The results show that FA pretreatment significantly enhances SCFAs production, resulting in a 4.5-fold increase compared to the control group. Mechanism investigations reveal that FA pretreatment accelerates PS solubilization, destroys EPS integrity, and increases easily biodegradable substrates in the fermentation broth. FA also inhibits methane production, leading to further SCFAs accumulation. The conversion of NH4+-N released during fermentation into FA facilitates the transition of wastewater treatment plants operation from linear to circular mode.

JOURNAL OF CLEANER PRODUCTION (2023)

Article Nanoscience & Nanotechnology

Halogen Doping Mechanism and Interface Strengthening in the Na3SbS4 Electrolyte via Solid-State Synthesis

Liangliang Yu, Jingxuan Yin, Chengwei Gao, Changgui Lin, Xiang Shen, Shixun Dai, Qing Jiao

Summary: In this study, a series of halogen-doped Na3SbS4 samples were synthesized using the solid-state method, and the relationship between crystal structure and Na+ ion conductivity was investigated through X-ray diffraction and Raman spectroscopy. The symmetric sodium battery assembled with the Na2.85SbS3.85Br0.15 electrolyte showed stable cycling for over 100 hours at room temperature with a current density of 0.1 mA/cm(2). This research provides a method to manufacture novel solid sodium electrolytes by exploring the effect of halogen doping in Na3SbS4.

ACS APPLIED MATERIALS & INTERFACES (2023)

Article Biochemistry & Molecular Biology

Two-Layered Biomimetic Flexible Self-Powered Electrical Stimulator for Promoting Wound Healing

Yining Chen, Wenxin Xu, Xin Zheng, Xuantao Huang, Nianhua Dan, Meng Wang, Yuwen Li, Zhengjun Li, Weihua Dan, Yunbing Wang

Summary: A two-layered self-powered electrical-stimulator-based wound dressing (SEWD) was designed, which integrated bionic tree-like piezoelectric nanofibers and adhesive hydrogel with biomimetic electrical activity. The SEWD showed good mechanical properties, adhesion properties, self-powered properties, high sensitivity, and bio-compatibility. In vitro and in vivo experiments demonstrated that SEWD converts mechanical energy into electricity to stimulate cell proliferation and wound healing.

BIOMACROMOLECULES (2023)

Article Agriculture, Multidisciplinary

Identification of Key Lipogenesis Stages and Proteins Involved in Walnut Kernel Development

Feng Jin, Ye Zhou, Pu Zhang, Ruimin Huang, Wei Fan, Baoxin Li, Guangzhu Li, Xiaobo Song, Dong Pei

Summary: This study investigated the development and accumulation of oil in walnut kernels. The researchers found that the oil content and oil bodies increased during the development of the kernels, especially in the early stages. They also identified key genes and proteins involved in fatty acid synthesis and oil body formation. These findings provide important insights into the molecular mechanism of oil biosynthesis in walnuts and potential strategies for genetic improvement.

JOURNAL OF AGRICULTURAL AND FOOD CHEMISTRY (2023)

Article Electrochemistry

Electrochemical Sensor Based on Co-Doped FePS3 Nanosheets for Ultra-Sensitive Detection of Dopamine in Human Serum

Wei Shan, Xiuyun Ma, Guobo Chen, Feicui Xu, Haizhou Zhao, Lei Dong, Xuefeng Yan, Zhaoshun Bi, Liangmin Yu, Meng Qiu

Summary: Electrochemical dopamine (DA) sensors have gained importance in the early diagnosis of psychiatric disorders due to their fast response, simplicity, and portability. However, traditional electrode modification materials have limitations such as high cost and low conductivity. Two-dimensional sulfide materials have high surface area and electrocatalytic properties, but their poor electroconductibility limits the detection signal. This paper introduces Co-doped FePS3 nanosheets for DA detection, which exhibited promising results in terms of detection limit, linear range, recovery, and stability in human serum samples.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2023)

Article Chemistry, Applied

Multi-scale structure and digestive property of bran starch in different particle size wheat bran

Yang Li, Haoran Wang, Lijuan Wang, Ju Qiu, Zaigui Li, Lili Wang

Summary: In this study, the structure and digestive property of starch isolated from wheat bran of different particle size were investigated and compared with wheat flour starch. Results showed that cell-scale milling caused significant destruction of crystalline regions and double helix, and increase in starch digestibility. Wheat bran starch had more resistant starch and lower digestibility compared to wheat flour starch, which were highly correlated with its thinner lamellas, more double helix proportion and compact fractal. This study contributes to the application of bran starch and highlights the effect of supramolecular structure on bran starch digestibility.

FOOD CHEMISTRY (2023)

Article Computer Science, Information Systems

Scarce Resource Dimensional Sentiment Analysis Using Domain-Distilled BERT

Wei Lin, Liang-Chih Yu

Summary: This study proposes a domain-distilled method to address the data scarcity problem in dimensional sentiment analysis. By using a domain discriminator to distinguish feature domains and maximizing the prediction loss, the proposed method improves the ability to learn domain-invariant features. Experimental results show that the proposed domain-distilled BERT outperforms the original BERT and other deep learning models in predicting dimensional sentiment scores.

JOURNAL OF INFORMATION SCIENCE AND ENGINEERING (2023)

Article Agricultural Engineering

EMISSIONS OF GREENHOUSE GASES AND AMMONIA FROM A WHEAT SITE UNDER INTENSIVE MANAGEMENT AFFECTED BY DIFFERENT FERTILIZATION PRACTICES

Zhongkai Zhou, Siyu Zhang, Na Jiang, Haifang Zhang, Lili Wang, Weiming Xiu, Jianning Zhao, Dianlin Yang

Summary: addressing the issue of greenhouse gas and ammonia emissions in wheat fields, the study evaluated the impact of different fertilization practices on soil emissions. The results showed that the use of organic and inorganic fertilizers together increased soil carbon and nitrogen levels, while reducing emissions of greenhouse gases and ammonia.

JOURNAL OF THE ASABE (2023)

Article Electrochemistry

Effect of ammonium fluoride concentration on synthesis of Co3O4/CC as cathode material for zinc cobalt battery applications

Wenhai Tan, Youfeng Zhang, Yichen Zhang, Yanbo Ma, Chao Zhao, Yinling Wang

Summary: This study synthesized Co3O4/CC cathode materials with excellent performance for aqueous zinc-ion batteries by varying the reactant concentration. The Co3O4/CC nanowires exhibited uniform distribution, regular surface, and small size on the carbon cloth. The battery assembled with Co3O4/CC material synthesized at a reactant concentration ratio of 2:1 showed better performance, with high discharge specific capacity and capacity retention rate.

INTERNATIONAL JOURNAL OF ELECTROCHEMICAL SCIENCE (2024)

Article Electrochemistry

Electro-osmotic impact of Williamson fluid flow induced by cilia curved walls

T. Salahuddin, Iqra Kousar, Mair Khan, M. Munawwar Iqbal Ch

Summary: This paper investigates the dynamics of fluid motion powered by cilia within a curved channel and examines the chemical reactions occurring in the presence of electro-osmotic impact. The findings offer insights into various flow characteristics and present a method for simulating non-Newtonian fluid models in three dimensions. Additionally, the model has potential applications in the development of micro-vascular chips, which could be crucial for diagnosing blood-related issues.

INTERNATIONAL JOURNAL OF ELECTROCHEMICAL SCIENCE (2024)

Review Electrochemistry

A critical review of enhanced soil electrokinetics using perforated electrodes, pipes, and nozzles

Ahmed Abou-Shady

Summary: Soil electrokinetic (SEK) is a significant technology with various applications in fields such as soil remediation, pollutant removal, and water regulation. This review summarizes the recent advancements in SEK, focusing on electrode modifications and material additives, and suggests future research directions.

INTERNATIONAL JOURNAL OF ELECTROCHEMICAL SCIENCE (2024)