期刊
INORGANIC CHEMISTRY
卷 57, 期 14, 页码 8033-8036出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.8b01044
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资金
- National Natural Science Foundations of China [21561020, 21661020, 21663016]
- Jiangxi Province [20153BCB23021]
The Bronsted basicity in activated metal organic framework-808 (hereinafter denoted as MOF-808a) was confirmed by the analyses of CO2-TPD-MS, in situ DRIFTS, and acid base titration. MOF-808a exhibited efficient recyclable catalytic activities for Heck coupling and oxidation of alcohol as a one-pot tandem reaction in base-free catalysis. It is the first evidence of the Bronsted basicity in zirconium metal organic frameworks (Zr-MOFs) and gave rise to a new opportunity to extend the catalytic application of Zr-MOFs.
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