期刊
ENERGIES
卷 11, 期 4, 页码 -出版社
MDPI
DOI: 10.3390/en11040999
关键词
glass platelets; composite separator; high-temperature stability; full-cell configuration cycling tests; lithium-ion battery
资金
- BayNW project ACoS [PTJ-1308-0002]
- TechnologieAllianzOberfranken (TAO)
- German Research Foundation (DFG)
- University of Bayreuth
A new type of high-temperature stable and self-supporting composite separator for lithium-ion batteries was developed consisting of custom-made ultrathin micrometer-sized glass platelets embedded in a glass fiber nonwoven together with a water-based sodium alginate binder. The physical and electrochemical properties were investigated and compared to commercial polymer-based separators. Full-cell configuration cycling tests at different current rates were performed using graphite and lithium iron phosphate as electrode materials. The glass separator was high-temperature tested and showed a stability up to at least 600 degrees C without significant shrinking. Furthermore, it showed an exceptional wettability for non-aqueous electrolytes. The electrochemical performance was excellent compared to commercially available polymer-based separators. The results clearly show that glass platelets integrated into a glass fiber nonwoven performs remarkably well as a separator material in lithium-ion batteries and show high-temperature stability.
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