期刊
DALTON TRANSACTIONS
卷 47, 期 33, 页码 11420-11428出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8dt01711e
关键词
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资金
- Natural Science Foundation of China [50972060]
- Weapon Research Support Fund [62201070804]
- Qing Lan Project
- Environmental Protection Scientific Research Project of Jiangsu Province [2016056]
- National Key R&D Program of China [2016YFB0302800]
- Basic Product Innovation Technology Research Project of Explosives
AgI/Bi5O7I plate composite was fabricated at room temperature by the phase transition and morphological transformation of BiOI microspheres. The orange BiOI microsphere was transferred to light yellow AgI/Bi5O7I plate by the addition of NaOH and AgNO3 to the system. The formation process and possible transformation mechanism of AgI/Bi5O7I plate were detected and are discussed. The visible light absorption area of AgI/Bi5O7I extended to 667 nm and photo-excited electrons migrated from Bi5O7I to AgI to effectively inhibit the recombination of photo-generated carriers in the Z-scheme AgI/Bi5O7I plate. As a result, the photocatalytic ability of AgI/Bi5O7I plate increased by a factor of 21.9 than that of pure Bi5O7I and a factor of 45.7 than that of pure AgI under visible light irradiation. This study provides a facile fabrication of Z-scheme visible light photocatalysts with high performance and a method for designing semiconductor photocatalysts with controllable morphology.
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