期刊
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
卷 541, 期 -, 页码 188-194出版社
ELSEVIER
DOI: 10.1016/j.colsurfa.2018.01.023
关键词
Fe2O3; QDs; 2D-C3N4; Photocatalytic degradation; High stability
资金
- National Nature Science Foundation of China [21476097, 21776118, 21507046]
- Six talent peaks project in Jiangsu Province [2014-JNHB-014]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
0D/2D photocatalysts have aroused concern due to the high charge mobility. Herein, a 0D/2D structure is formed by employing a facile method to disperse Fe2O3 Quantum-Dots (QDs) on 2D-C3N4 without aggregation at a relatively low temperature of 200 degrees C. The ultrathin monolayer 2D structure, highly dispersed Fe2O3 QDs, the strong coupling as well as quantum-sized confinement effect between them lead to superior visible-light-driven photocurrent performance and photocatalytic activity. Particularly, the 0.5% Fe2O3 QDs/2D-C3N4 composite exhibits the highest photocatalytic activity under visible light. More importantly, the 0D/2D photocatalysts show superior durability with little photocatalytic activity decline in the circular reaction for the photocatalytic degradation of organic pollution. Therefore, this work supplies a new opportunity to construct multifunctional 0D/2D photocatalysts for degradation of pollutants in water.
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