期刊
CHINESE JOURNAL OF CHEMISTRY
卷 36, 期 4, 页码 329-332出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cjoc.201700750
关键词
solid reduction; subnanometer-sized clusters; gold catalysts; CO2 hydrogenation
资金
- National Natural Science Foundation of China [21676045, 21476226, 21203182, 21176037]
- National Key R&D Program of China [2016YFB0600902]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDB17020400]
- Dalian Science Foundation for Distinguished Young Scholars [2016RJ04]
- Youth Innovation Promotion Association CAS
- Natural Science Foundation of Liaoning Province [201602169]
An effective solvent-free method based on a solid-reduction process was developed to fabricate ultrafine gold catalysts. By this method we revealed a strong size-dependent activity of Au species in which subnanometer-sized clusters exhibited the best activity in the hydrogenation of CO2 to formate, with a turnover number of up to 9278 over 7 h at 90 degrees C.
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