期刊
CATALYSIS TODAY
卷 324, 期 -, 页码 90-96出版社
ELSEVIER
DOI: 10.1016/j.cattod.2018.06.013
关键词
Hydrogen production; Formic acid; Palladium nanoparticles; Carbon xerogels; Nitrogen doping
资金
- JST, PRESTO [JPMJPR1544]
- Japan Society for the Promotion of Science (JSPS) [26220911, 25289289, 26630409, 26620194]
- MEXT
- JSPS [A17F173810]
- University of Liege
- European Commission [600405]
- Walloon Region (project HYLIFE) [1410135]
- RFCS (PROMOTEE) [709741]
- Elemental Strategy Initiative to Form Core Research Center
- Walloon Region (project BATWAL) [1318146]
N-doped carbon xerogels synthesized from melamine-resorcinol-formaldehyde aqueous gels were used as supports for the preparation of Pd-based catalysts for the formic acid dehydrogenation reaction. The effect of the pore texture and nitrogen content of the carbon xerogels on the catalytic activity for the hydrogen production was investigated. It was observed that an appropriate nitrogen doping in a well-defined micro-mesoporous carbon xerogel enables the preparation of Pd catalysts with appreciable catalytic enhancement towards the formic acid dehydrogenation as compared to the N-free counterpart, reaching an initial TOF value of 2014 h(-1).
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