Article
Materials Science, Ceramics
Zheng Li, Jun Yang, Yan Xing, Chunlei Wan, Satoshi Watanabe, Wei Pan
Summary: Using density functional theory (DFT) method, the intrinsic lattice thermal conductivities of Ln(2)Sn(2)O(7)(Ln = La, Gd) were calculated, showing the significant role of optical phonons in lattice thermal conduction in rare-earth pyrochlore materials with contributions exceeding 50% and 64% in La(2)Sn(2)O(7) and Gd2Sn2O7, respectively.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2021)
Article
Chemistry, Physical
Bangzhi Ge, Hyungseok Lee, Chongjian Zhou, Weiqun Lu, Jiabin Hu, Jian Yang, Sung-Pyo Cho, Guanjun Qiao, Zhongqi Shi, In Chung
Summary: This study introduces a new strategy to control the thermal and charge transport properties of solids by designing desirable defect architecture. By introducing a high concentration of indium to CuFeS2, a stabilized and highly unusual local structure is formed, resulting in a significant reduction in lattice thermal conductivity. This approach achieves one of the highest thermoelectric figures of merit, ZT, among chalcopyrite sulfides.
Review
Materials Science, Multidisciplinary
Chuan-Dong Zhou, Bo Liang, Wen-Jie Huang, Jacques-Guillaume Noudem, Xiao-Jian Tan, Jun Jiang
Summary: This review summarizes the recent progress in studying phonon dispersion models and proposes using the modified sinusoidal phonon dispersion model for accurately determining lattice thermal conductivity. Furthermore, experimental methods that can reduce lattice thermal conductivity in thermoelectric materials are reviewed, such as methods that generate standing waves or anharmonic lattice vibrations. A high concentration of standing waves and anharmonic lattice vibrations can effectively suppress excessive lattice thermal conductivity. Finally, this review discusses the challenges of applying sinusoidal phonon dispersion to real materials, which are often complicated and time-consuming, especially when dealing with material defects.
Article
Materials Science, Multidisciplinary
B. Bommalingaiah, Narayan Gaonkar, R. G. Vaidya
Summary: Theoretical investigation of macroscopic polarization effects on lattice thermal conductivity of GaN reveals significant impact of polarization fields on thermal conductivity, especially from high frequency transverse mode phonons. Numerical calculations show good agreement with experimental reports for thermal conductivity of different dimension samples with and without polarization fields.
Article
Chemistry, Multidisciplinary
Fei Jia, Shuang Zhao, Jing Wu, Ling Chen, Te-Huan Liu, Li-Ming Wu
Summary: This study reports a unique ternary sulfide compound, Cu3BiS3, with ultralow thermal conductivity. By using DFT calculations and analysis, researchers found that the Cu atoms in Cu3BiS3 are coordinated in a two-dimensional triangular arrangement, leading to efficient out-of-plane phonon scattering and reduced thermal conductivity.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Physics, Applied
Zongwei Zhang, Honghao Yao, Xue Jia, Xinyu Wang, Xiaofang Li, Chen Chen, Xi Lin, Jiehe Sui, Xingjun Liu, Jun Mao, Guoqiang Xie, Qian Zhang
Summary: The study demonstrates that alignment of valence bands through alloying and doping can enhance the thermoelectric performance of zintl phases, with increased Seebeck coefficient and decreased lattice thermal conductivity achieved in CaCd2Sb2 through manipulation of valence band degeneracy.
APPLIED PHYSICS LETTERS
(2022)
Article
Materials Science, Multidisciplinary
X. Yang, A. Jena, F. Meng, S. Wen, J. Ma, X. Li, W. Li
Summary: In this study, the effect of electron-phonon interaction on the lattice thermal conductivity of graphene was investigated using first-principles calculations. It was found that the indirect coupling between flexural acoustic phonons and electrons has a significant impact on thermal conductivity in graphene, particularly due to the dominance of normal processes. Additionally, an unusual minimum thermal conductivity was observed at a specific charge carrier density in graphene.
MATERIALS TODAY PHYSICS
(2021)
Article
Materials Science, Multidisciplinary
Niuchang Ouyang, Chen Wang, Yue Chen
Summary: Through atomic-level investigations, we have discovered the phonon and thermal transport properties of strongly anharmonic alloy-based thermoelectric materials and revealed the correlation between the decreased thermal conductivity of SnS0.75Se0.25 and randomization of Se atoms.
MATERIALS TODAY PHYSICS
(2022)
Article
Materials Science, Multidisciplinary
Wenhao Sha, Xuan Dai, Siyu Chen, Binglun Yin, Fenglin Guo
Summary: Two-dimensional (2D) PbTe monolayers, known for their excellent physical properties, have attracted great attention as new thermoelectric materials. Understanding their thermal properties is crucial for practical applications. In this study, we developed a machine-learned potential specific for 2D PbTe monolayers using a neuroevolution potential model. By using this potential, we found an abnormal increase in thermal conductivity with increasing biaxial strain due to the enhancement of low-frequency phonons. These results can provide guidance for their practical use once validated experimentally.
MATERIALS TODAY PHYSICS
(2023)
Article
Materials Science, Multidisciplinary
Hanxia Zhang, Xiaoyu Yang, Xinyue Zhang, Pengfei Nan, Binghui Ge, Zhiwei Chen, Yanzhong Pei
Summary: Anisotropy in lattice thermal conductivity (KL) of crystals is commonly caused by the anisotropic crystal structure. However, this anisotropy can be easily eliminated in polycrystalline materials due to the random orientation of grains. In this study, a significant enhancement in KL-anisotropy is achieved in polycrystalline (GeTe)m(Bi2Te3)n through ordered 1D/2D defects induced by high-concentration vacancies. The resulting KL-anisotropy is approximately twice as large as that of GeTe. This research provides an effective strategy for manipulating the anisotropy of heat transport through a structural control of ordered high-dimension defects, which can be well described by a phonon-defect scattering model.
MATERIALS TODAY PHYSICS
(2023)
Article
Nanoscience & Nanotechnology
Chao Yang, Yong Luo, Yafen Xia, Teng Fang, Zhengliang Du, Xie Li, Jiaolin Cui
Summary: In this study, the electronic and phonon transports in Cu8GeSe6 compound were engineered by incorporating In2Te3 species, resulting in improved thermoelectric performance.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Chemistry, Multidisciplinary
Ke Wang, WuXing Zhou, Yuan Cheng, Min Zhang, Hai Wang, Gang Zhang
Summary: The study investigated how spin affects the phononic properties of CrI3 monolayers, finding that infrared spectra can be used to identify magnetic order and explaining the mechanisms behind thermal expansion coefficients and lattice thermal conductivity being influenced by magnetic phases. This research provides insights into spin-lattice coupling and highlights the potential of spintronic monolayers as thermal switching devices for active heat flow control.
Article
Materials Science, Multidisciplinary
H. K. Weng, A. Nagakubo, H. Ogi, H. Watanabe
Summary: This study evaluated the out-of-plane thermal conductivity and elastic constant of epitaxial [100] C-12/C-13 superlattice diamonds with different layer thicknesses. The results indicated that phonon transport in the synthesized superlattice specimens is governed by mass difference and not interfacial defects. Additionally, the study found that thermal conductivity is affected by the phonon group velocity and the mini-umklapp scattering effect in the superlattice.
Article
Chemistry, Multidisciplinary
Yirong Gao, Jianxing Huang, Jun Cheng, Shou-Hang Bo
Summary: By using Li-6 isotope substitution, we selectively changed the phonon properties associated with lithium without introducing additional defects or disorders. Our results showed that lower lithium vibration frequency results in higher ionic conductivity and lower activation energy. We also quantified the effect of lithium-related phonons on migration entropy and attempt frequency.
SCIENCE CHINA-CHEMISTRY
(2023)
Article
Nanoscience & Nanotechnology
Chao Yang, Yong Luo, Yafen Xia, Liangliang Xu, Zhengliang Du, Zhongkang Han, Xie Li, Jiaolin Cui
Summary: By alloying with gallium, the phase transformation in the argyrodite compound can be eliminated, extending its high-temperature cubic phase range and improving its thermoelectric performance. The power factor increases, and the lattice thermal conductivity decreases as a result.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Thermodynamics
Shuo Jin, Zhongwei Zhang, Yangyu Guo, Jie Chen, Masahiro Nomura, Sebastian Volz
Summary: By combining molecular dynamics simulations and machine learning techniques, this study systematically investigates the optimization of interfacial thermal transport in Si/Ge heterostructures through interfacial nanostructuring. The results show that the interfacial thermal resistance significantly depends on interfacial nanostructures, providing diverse guidance for optimization.
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER
(2022)
Article
Chemistry, Physical
Jia He, Yanxiao Hu, Dengfeng Li, Jie Chen
Summary: The study shows that fluorination and chlorination can stabilize alpha'-borophene and maintain its semiconductor nature. When hydrogen is replaced with fluorine or chlorine, a significant reduction in thermal conductivity is observed, attributed to the weakening of B-B bonds and softening of phonon modes. As a result, chlorinated alpha'-borophene exhibits a high thermoelectric figure of merit along the armchair direction at 300 K.
Article
Nanoscience & Nanotechnology
Xiaoyi Peng, Pengfei Jiang, Yulou Ouyang, Shuang Lu, Weijun Ren, Jie Chen
Summary: This study investigates the effect of interfacial superlattice structures on the Kapitza resistance between a graphene/water interface through molecular dynamics simulations. The results show that introducing interfacial superlattices can significantly reduce the Kapitza resistance. The analysis suggests that this improvement is mainly due to the enhanced phonon scattering rate in the interfacial graphene layer, which increases the thermal resistance between the graphene layer and its neighboring layer.
Article
Physics, Multidisciplinary
Zhongwei Zhang, Yangyu Guo, Marc Bescond, Jie Chen, Masahiro Nomura, Sebastian Volz
Summary: Understanding and quantifying the coherence of thermal excitations is an important problem in physics. The traditional phonon gas model fails to capture this coherence. In this study, a new heat conduction formalism is proposed that combines the phonon gas model and the wave nature of thermal phonons. The theory and simulations reveal two types of coherence in different temperature ranges.
PHYSICAL REVIEW LETTERS
(2022)
Article
Physics, Applied
Cuiqian Yu, Yanxiao Hu, Jia He, Shuang Lu, Dengfeng Li, Jie Chen
Summary: Recently, the important role of high-order anharmonic phonon-phonon interactions has been revealed in several materials. By solving the Boltzmann transport equation, the significant impact of four-phonon scattering on thermal transport in honeycomb structured monolayer BAs and its hydrogenated bilayer counterparts has been shown. After considering four-phonon scattering, the lattice thermal conductivity of all these structures is reduced, especially for monolayer BAs, which shows a huge drop of 80% mainly due to the suppression of phonon lifetimes. In contrast to graphene, the thermal conductivity of monolayer BAs is abnormally lower than its bilayer counterparts, attributed to the much larger phonon scattering rate. The contribution of flexural acoustic phonon exhibits the most significant reduction in both monolayer and bilayer BAs with horizontal mirror symmetry after including four-phonon scattering.
APPLIED PHYSICS LETTERS
(2022)
Review
Physics, Multidisciplinary
Jie Chen, Xiangfan Xu, Jun Zhou, Baowen Li
Summary: Interfacial thermal resistance (ITR) is a major obstacle for heat transfer between materials, and understanding it is crucial for efficient heat dissipation in electronic and photonic devices, batteries, etc. This comprehensive review examines ITR, focusing on theoretical, computational, and experimental developments over the past 30 years. It covers fundamental theories, computational methods, and experimental tools for probing ITR, as well as challenges and opportunities in studying nanoscale and atomic scale interfaces.
REVIEWS OF MODERN PHYSICS
(2022)
Article
Chemistry, Multidisciplinary
Jianhui Jiang, Shuang Lu, Yulou Ouyang, Jie Chen
Summary: This paper explores the origin of the convergence of thermal conductivity in two-dimensional materials and reveals the important role of the normal scattering process in determining the thermal conductivity of these materials.
Article
Physics, Multidisciplinary
Ming-Jun Li, Lina Yang, Deng Wang, Si-Yi Wang, Jing-Nan Tang, Yi Jiang, Jie Chen
Summary: Traditional methods cannot non-destructively and quickly detect the internal structure of pavements, so it is important to accurately and quickly predict the mechanical properties of layered pavements. In recent years, machine learning has shown great superiority in solving nonlinear problems. This paper proposes a method based on random forest regression to predict the maximum deflection and damage factor of layered pavements under instantaneous large impact using the deflection basin parameters obtained from falling weight deflection testing. The prediction results have high consistency with finite element simulation results, indicating the potential of this method in non-destructive evaluation of pavement structure.
Article
Materials Science, Multidisciplinary
Wei-Jun Ren, Shuang Lu, Cui-Qian Yu, Jia He, Jie Chen
Summary: The carbon honeycomb structure has both high in-plane thermal conductivity and high axial thermal conductivity, which is robust to structural disorder. This study suggests that the carbon honeycomb structure has unique advantages to serve as a thermal management material.
Article
Physics, Multidisciplinary
Jian-Hui Jiang, Shuang Lu, Jie Chen
Summary: The rise of artificial microstructures has allowed for the modulation of various waves, including light, sound, and heat. In this study, we propose an atomic level triangular structure in single-layer graphene to achieve the phonon focusing effect. Our simulation results demonstrate that the height of the triangular structure can control multiple features related to the phonon focusing effect in the positive incident direction. Additionally, a distinct focusing pattern and enhanced energy transmission coefficient are observed in the reverse incident direction. Fourier transform analysis provides insights into the mode conversion physics of the phonon wave packet.
CHINESE PHYSICS LETTERS
(2023)
Article
Physics, Applied
Weijun Ren, Shuang Lu, Cuiqian Yu, Jia He, Zhongwei Zhang, Jie Chen, Gang Zhang
Summary: In this study, non-equilibrium molecular dynamics simulations were used to investigate the in-plane thermal conductivity of graphene/hexagonal boron nitride (h-BN) moire superlattices. It was found that the in-plane thermal conductivity decreases monotonically with increasing interlayer rotation angle within a small range. The atomic stress amplitude exhibits a periodic distribution corresponding to the structural moire pattern. The analysis at the atomic level revealed a competition between the magnitude and directional change of the in-plane heat flow, with the directional change playing a dominant role in determining the in-plane thermal conductivity. The decreasing trend of in-plane thermal conductivity at small rotation angles was explained by the reduced low-frequency phonon transmission and the blue shift of the transmission peak.
APPLIED PHYSICS REVIEWS
(2023)
Article
Materials Science, Multidisciplinary
Zhongwei Zhang, Yangyu Guo, Marc Bescond, Masahiro Nomura, Sebastian Volz, Jie Chen
Summary: In this paper, a theoretical model for exploring phonon coherence based on spectroscopy is proposed and validated using Brillouin light scattering data and molecular dynamic simulations. The model shows that confined modes exhibit wavelike behavior with a higher ratio of coherence time to lifetime. The spectroscopy data also demonstrates the dependence of phonon coherence on system size. The proposed model allows for reassessing conventional spectroscopy data to obtain coherence times, which are crucial for understanding and estimating phonon characteristics and heat transport in solids.
Article
Materials Science, Multidisciplinary
Cuiqian Yu, Shuyue Shan, Shuang Lu, Zhongwei Zhang, Jie Chen
Summary: Through molecular dynamics simulations, the fundamental characteristics of second sound are explored in a transient heat conduction modeling in single-layer and multilayer graphene and graphite. The results demonstrate that second sound can carry more heat energy and maintain for a longer lifetime than ballistic pulse. The effects of thickness and temperature on second sound propagation are also investigated.
Article
Materials Science, Multidisciplinary
Shuang Lu, Weijun Ren, Jia He, Cuiqian Yu, Pengfei Jiang, Jie Chen
Summary: Introduced the importance of crystal symmetry in thermal transport in solids, focusing on the case of inversion symmetry breaking in monolayer Ta2CS2 that abnormally enhances lattice thermal conductivity in 2D functionalized MXenes.
Article
Materials Science, Multidisciplinary
Yulou Ouyang, Cuiqian Yu, Jia He, Pengfei Jiang, Weijun Ren, Jie Chen
Summary: In this study, the machine learning potential (MLP) and molecular dynamics simulations were used to predict the thermal conductivity (kappa) and assess the effect of anharmonicity on thermal transport properties of cubic boron arsenide (BAs) and diamond. The MLP based on the matrix tensor algorithm accurately described the lattice dynamics behaviors in both materials. The phonon spectral energy density analysis showed that MLP effectively captured the anharmonicity-induced phonon mode softening and linewidth broadening. Results demonstrated that the accuracy of MLP in predicting kappa was comparable to that of density-functional theory calculations for diamond and BAs. However, high-order phonon scattering process had a significant impact on BAs, leading to the overestimation of kappa compared to experimental results. Equilibrium molecular dynamics simulations combined with MLP provided accurate predictions of kappa for both BAs and diamond. The study suggested that molecular dynamics simulation combined with MLP is a reliable and computationally efficient tool for predicting material's thermal conductivity.
Article
Chemistry, Physical
Jie Sheng, Jingshan He, Dun Ma, Yuanbo Wang, Wu Shao, Tian Ding, Ronghao Cen, Jingwen He, Zhihao Deng, Wenjun Wu
Summary: This study presents an innovative approach to improve the photovoltaic conversion characteristics and stability of perovskite solar cells through carbon electrode interface modification. By in-situ polymerization and carbonization on the surface of nano-graphite, a dendritic structure carbon electrode is formed, reducing the work function and aligning the energy levels with perovskite. This leads to improved charge and hole collection efficiency, resulting in increased photovoltaic conversion efficiency. Furthermore, the modified carbon electrode-based perovskite solar cells exhibit exceptional stability, maintaining high efficiency even without encapsulation.
Article
Chemistry, Physical
Guodong Shi, Jian Song, Xiaoxiao Tian, Tongtong Liu, Zhanjun Wu
Summary: This study demonstrates the improvement of mechanical properties and reduction of coefficient of thermal expansion (CTE) in graphene oxide (GO)/epoxy (EP) nanocomposites by enhancing the interface between GO and EP through functionalization and incorporating rigid-flexible interphases. The results reveal that the SiO2-PEA-GO hybrid exhibits better strengthening and toughening effects, as well as lower CTE, compared to the PEA-GO hybrid due to the presence of rigid-flexible interfaces with higher bonding strength and better energy dissipation mechanisms. Additionally, the nanocomposites with longer polyetheramine (PEA) molecules in the rigid-flexible interphases demonstrate higher strength and toughness, while maintaining a lower CTE. This work provides a promising strategy for constructing adjustable flexible-rigid interfacial structures and offers potential in developing GO/EP nanocomposites with high mechanical properties and low CTE.
Article
Chemistry, Physical
Rafal Janus, Sebastian Jarczewski, Jacek Jagiello, Piotr Natkanski, Mariusz Wadrzyk, Marek Lewandowski, Marek Michalik, Piotr Kustrowski
Summary: In this study, a facile procedure for the synthesis of CMK-1 and CMK-2 carbon replicas was developed. The method utilizes basic laboratory equipment and a renewable carbon source, and operates under mild conditions. The resulting carbon mesostructures exhibit exquisite replication fidelity and structural homogeneity, making them suitable for applications in various fields.
Article
Chemistry, Physical
Anqi Wang, Connor J. MacRobbie, Alex Baranovsky, Jean-Pierre Hickey, John Z. Wen
Summary: In this study, a novel polymer-free nanothermite aerogel with a wide range of nanoparticle loading was fabricated via a new additive manufacturing process. The SEM images showed a unique porous structure formed by extra thin rGO sheets, wrapping individual nanothermite clusters. The DSC-TGA results and high-speed combustion videos confirmed the enhanced energetic performance of the printed specimen.
Article
Chemistry, Physical
Wanze Wu, Misheng Zhao, Shiwei Miao, Xiaoyan Li, Yongzhong Wu, Xiao Gong, Hangxiang Wang
Summary: Superhydrophobic solar-driven interfacial evaporator is an energy-efficient technology for seawater desalination, which is easily fabricated using robust photothermal superhydrophobic coating and substrate. The created bifunctional coating on the melamine sponge substrate shows stable and highly efficient photothermal and superhydrophobic performance for seawater desalination. This superhydrophobic solar-driven interfacial evaporator is expected to have wide applications in seawater desalination.
Article
Chemistry, Physical
Zichen Xiang, Zhi Song, Tiansheng Wang, Menghang Feng, Yijing Zhao, Qitu Zhang, Yi Hou, Lixi Wang
Summary: This study presents a co-electrospinning synthesis strategy to fabricate lightweight and porous Co@C composite nanofibres with wideband microwave attenuation capacity. The addition of MOF-derived Co additives enhances the low-frequency absorption performance.
Article
Chemistry, Physical
J. Snow, C. Olson, E. Torres, K. Shirley, E. Cazalas
Summary: This study investigates the use of a perovskite-based graphene field effect transistor (P-GFET) device for X-ray detection. The sensitivity and responsivity of the device were found to be influenced by factors such as X-ray tube voltage, current, and source-drain voltage. Simulation experiments were conducted to determine the dose rate and energy incident on the device during irradiation.
Article
Chemistry, Physical
Zuzana Jankovska, Lenka Matejova, Jonas Tokarsky, Pavlina Peikertova, Milan Dopita, Karolina Gorzolkova, Dominika Habermannova, Michal Vastyl, Jakub Belik
Summary: This study provides new insights into microwave-assisted pyrolysis of scrap tyres, demonstrating that it can produce microporous carbon black with potential application in xylene adsorption. Compared to conventional pyrolysis, microwave pyrolysis requires less time and energy while maintaining similar adsorption capacity.
Article
Chemistry, Physical
Max Bommert, Bruno Schuler, Carlo A. Pignedoli, Roland Widmer, Oliver Groning
Summary: A detailed understanding of the interaction between molecules and two-dimensional materials is crucial for incorporating functional molecular films into next-generation 2D material-organic hybrid devices. This study compares the energy level alignment of different-sized fullerenes on a Moire superstructure and finds that C-84 fullerenes can be either neutral or negatively charged depending on slight variations of the electrostatic potential. This discovery suggests a new path to achieve ambipolar charge transfer without overcoming the electronic gap of fullerenes.
Article
Chemistry, Physical
Yuanjing Cheng, Xianxian Sun, Ye Yuan, Shuang Yang, Yuanhao Ning, Dan Wang, Weilong Yin, Yibin Li
Summary: The dual-structure aerogel (GS) consisting of flexible silica fibers and graphene honeycomb structures exhibits excellent resilience, flexibility, and reliability. It also shows remarkable wave absorbing performance, making it an ideal candidate for microwave absorption applications such as flexible electronics and aerospace.
Article
Chemistry, Physical
Shuyu Fan, Yinong Chen, Shu Xiao, Kejun Shi, Xinyu Meng, Songsheng Lin, Fenghua Su, Yifan Su, Paul K. Chu
Summary: Graphene coatings are promising solid lubrication materials due to their mechanical properties. This study presents a new method for in situ deposition of high-quality graphene coatings on hard substrates using NiCo solid solution and competitive reaction strategies. The graphene coating deposited on substrates with deep NiCo solid solution demonstrates superior low-friction and durability.
Article
Chemistry, Physical
Mengdi Wang, Sanyin Qu, Yanling Chen, Qin Yao, Lidong Chen
Summary: The improved thermoelectric properties of conducting polymers are achieved by selectively capturing single-walled carbon nanotubes (SWNTs) in a conducting polymer film, leading to increased carrier mobility and reduced thermal conductivity. The resulting composite film exhibits significantly higher electrical conductivity and lower thermal conductivity compared to films with a mixture of SWNTs. This work provides a convenient and efficient method to enhance the thermoelectric properties of conducting polymers.
Review
Chemistry, Physical
Heng Wei, Weihua Li, Kareem Bachagha
Summary: This article reviews the research progress of carbon nanotube-based microwave absorbing materials (MAMs) in recent years, covering the fundamental theory, design strategies, synthesis methods, and future development directions.
Article
Chemistry, Physical
Chenguang Shi, Junlong Huang, Zongheng Cen, Tan Yi, Shaohong Liu, Ruowen Fu
Summary: This study developed a high-performance Li metal host material, which achieved dendrite-free Li deposition with a low nucleation overpotential and high Coulombic efficiencies through the combination of Ti3C2-g-PV4P sheets and Ag nanoparticles. The full cells assembled with the Li@host anode and LiFePO4 cathode exhibited high discharge capacity and excellent cycling stability, demonstrating a perspective design for future energy storage devices.
Article
Chemistry, Physical
Tomotaro Mae, Kentaro Kaneko, Hiroki Sakurai, Suguru Noda
Summary: A new partial prelithiation method for SiO/C-CNT electrodes was developed, which showed reduced irreversible capacity and achieved high energy densities with good reversibility. The method allows for precise control of the degree of prelithiation and is applicable to various chemistries.