Article
Chemistry, Physical
Xinyue Liu, Weinan Tang, Shujie Liu, Xiong Chen, Yupeng Li, Xiaoying Hu, Liang Qiao, Yi Zeng
Summary: The research focuses on exploring the potential of using graphdiyne (GDY) as a promising substrate for single atom catalysts (SACs) in CO oxidation reactions. The study reveals that CO adsorption on Ni-GDY or co-adsorption of CO and O-2 on Cu-GDY is more favorable than O-2 adsorption, leading to a preference for CO oxidation starting with the LH reaction with a lower energy barrier.
APPLIED SURFACE SCIENCE
(2021)
Article
Chemistry, Physical
Xilin Zhang, Wenli Kang, Xiaodong Li, Qianqian Peng, Zongxian Yang, Weichao Wang
Summary: This study systematically explores the catalytic properties of a single Pt atom supported on PtS2, PtSe2, PtTe2 for CO oxidation. The results show that Pt1/PtTe2 exhibits the highest activity and provides an important reference for the design of SACs based on TMDs.
APPLIED SURFACE SCIENCE
(2023)
Article
Chemistry, Physical
Shuaihao Tang, Liang Xu, Bojun Peng, Feilong Xiong, Tong Chen, Xin Luo, Xin Huang, Haotian Li, Jian Zeng, Zongle Ma, Ling-Ling Wang
Summary: This study systematically investigated the effect of Ga doping on the performance of Pd/CeO2 SACs system using DFT calculations and transition state theory. Ga doping significantly enhanced the stability of Pd single atoms and promoted the catalytic performance of the CO oxidation reaction effectively. This work provides a new perspective for SACs modification.
APPLIED SURFACE SCIENCE
(2022)
Article
Chemistry, Physical
Ya-Qiong Su, Yan-Yang Qin, Tiantian Wu, De-Yin Wu
Summary: Single-atom catalysis is a hot topic in heterogeneous catalysis, but determining the stability and activity of single atoms on oxide supports compared to clusters and nanoparticles remains challenging. It was found that single Au atoms at step-edges serve as active sites for low-temperature CO oxidation, and the interface between Au nanoparticles and CeO2 can directly catalyze CO oxidation through the Mars-van Krevelen mechanism.
JOURNAL OF CATALYSIS
(2022)
Article
Chemistry, Physical
Zhenwei Zhang, Liang Zhang, Xiaoyang Wang, Yuan Feng, Xiangwen Liu, Wenming Sun
Summary: This study systematically investigates the potential of gamma-graphyne as a substrate for metal catalysts in different concentration modes for CO oxidation. The results show that single-atom Co, Ir, Rh, and Ru, as well as dual-atom Rh-2/GY, exhibit high activity in oxidizing CO molecules.
Article
Chemistry, Physical
Yang Chen, Qiang Wan, Liru Cao, Zhe Gao, Jian Lin, Lin Li, Xiaoli Pan, Sen Lin, Xiaodong Wang, Tao Zhang
Summary: This study reveals the dependence of Pt single atoms' electronic structure on the facets of CeO2 and demonstrates the impact of such dependence on catalytic performance. By controlling the electron transfer patterns of Pt-O-Ce microstructures, the positively charged or metallic states of Pt single atoms can be achieved, resulting in enhanced complete oxidation of CO and activation of H2, respectively.
JOURNAL OF CATALYSIS
(2022)
Article
Chemistry, Applied
Chun Zhu, Jin-Xia Liang, Yang-Gang Wang, Jun Li
Summary: MXenes have garnered significant attention for their versatile and excellent physicochemical properties, particularly for their potential applications as robust supports for single-atom catalysts. In this study, quantum chemical investigations using density functional theory were conducted to systematically examine the geometries, stability, and electronic properties of oxygen-functionalized Ti2C (Ti2CO2)-supported single-atom catalysts M-1/Ti2CO2 (M = Fe, Co, Ni, Cu, Ru, Rh, Pd, Ag, Os, Ir, Pt, Au). Among the transition metals in groups 8-11, a new non-noble metal single-atom catalyst Fe-1/Ti2CO2 was found to exhibit excellent catalytic performance for low-temperature CO oxidation. Detailed analysis revealed that O-2 and CO adsorption on the Fe-1 atom of Fe-1/Ti2CO2 is favorable. Furthermore, five possible mechanisms for CO oxidation on this catalyst, including Eley-Rideal, Langmuir-Hinshelwood, Mars-van Krevelen, Termolecular Eley-Rideal, and Termolecular Langmuir-Hinshelwood (TLH) mechanisms, were evaluated. Based on the calculated reaction energies for different pathways, it was observed that Fe-1/Ti2CO2 demonstrates excellent kinetics for CO oxidation via the TLH mechanism, featuring a significantly low energy barrier (0.20 eV) for the rate-determining step. These findings establish Fe-1/Ti2CO2 MXene as a highly promising 2D material for constructing robust non-noble metal catalysts.
CHINESE JOURNAL OF CATALYSIS
(2022)
Article
Chemistry, Physical
Qi Wang, Juhui Gong, Heng Zhang, Qi-Yuan Fan, Lei Xue, Jinfang Wu, Jiaxin Li, Yan Wang, Ze Liu, Rui Gao, Shanghong Zeng
Summary: This study reports a co-promotion strategy of PtCu single-atom alloy and copper-ceria interface for preferential oxidation of CO. The Pt0.1Cu0.19/CeO2 catalyst exhibits superior catalytic performance and excellent stability, attributed to the regulation of the electronic interaction between Pt and Cu as well as the high proportion of oxygen vacancies.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2022)
Article
Chemistry, Multidisciplinary
Anuj Kumar, Dipak Kumar Das, Raj Kishore Sharma, Manickam Selvaraj, Mohammed A. Assiri, Saira Ajmal, Guoxin Zhang, Ram K. Gupta, Ghulam Yasin
Summary: In this study, density functional theory calculations were used to investigate the activity and mechanism of binuclear phthalocyanine (bN-Pc) models combined with Fe and Co for the oxygen reduction reaction (ORR) in alkaline media. The results showed that Fe-Co-bN-Pc exhibited stronger ORR performance with a lower energy barrier. This research provides a scientific and engineering perspective for the construction of dual-atom active sites in future ORR electrocatalysts.
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY
(2023)
Article
Chemistry, Physical
Jiaojiao Song, Yixuan Yang, Shoujie Liu, Lei Li, Nan Yu, Yuteng Fan, Zhiming Chen, Long Kuai, Baoyou Geng
Summary: This study investigates the impact of dispersion and support on the activity of Pt in CO oxidation reaction, revealing that reducible TiO2 significantly influences Pt activity with lower apparent activation barriers, and that single-atom dispersion of Pt maximizes active sites.
Article
Chemistry, Physical
Pei Zhu, Wen-Xiong Shi, Ying Wang, Zhi-Ming Zhang, Lina Li, Changhua An
Summary: A novel polymerization-sulfurization-pyrolysis strategy was used to construct N,S co-doped carbon to anchor Co single atom (Co-SAs) catalysts for the selective electro-oxidation of thioethers in acidic solution. The as-obtained Co-SAs showed excellent electrocatalytic activity and stability, outperforming commercial Pt electrode and state-of-the-art catalysts. The high performance of Co-SAs was attributed to the Co-S2N4 coordination geometry, which significantly promoted desorption of the products.
Article
Chemistry, Physical
Pei Zhu, Wen-Xiong Shi, Ying Wang, Zhi-Ming Zhang, Lina Li, Changhua An
Summary: Researchers have successfully synthesized N, S co-doped carbon with 10% cobalt single atomic sites (Co-SAs/NSC) through a novel polymerization-sulfurization-pyrolysis strategy. The Co-SAs/NSC material exhibits excellent electrocatalytic activity and stability for the selective electro-oxidation of thioethers in acidic solution. This work provides a convenient strategy for the development of high-performance single-atom catalysts for the resourceful utilization of sulfur-containing pollutants.
Article
Chemistry, Physical
San Hua Lim, Chee Kok Poh
Summary: This study demonstrates that SiC monolayers are promising substrates for the development of highly stable single atom catalysts, with enhanced diffusion barrier energy and stability. These catalysts also show a significant reduction in activation barrier energy for CO oxidation.
Article
Chemistry, Physical
Xiaoqin Feng, Jingchun Su, Chenglei Yan, Guibin Chen, Qingming Deng
Summary: Based on density functional theory (DFT) calculations, we found that Sc-SP single atom catalyst exhibits the highest catalytic activity for CO oxidation, and its catalytic behavior is independent of different macrocyclic ligands. This provides a new strategy for designing efficient single atom catalysts.
APPLIED SURFACE SCIENCE
(2023)
Article
Chemistry, Physical
Mingming Luo, Zhao Liang, Chao Liu, Xiaopeng Qi, Mingwei Chen, Rizwan Ur Rehman Sagar, Hui Yang, Tongxiang Liang
Summary: The study demonstrates that Mn and N co-doped single-vacancy graphene exhibits superior catalytic performance for CO oxidation through both TER and LH mechanisms, providing a theoretical basis for the development of efficient and low-cost catalysts to oxidize CO at room temperature.
APPLIED SURFACE SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Shamraiz Hussain Talib, Zhansheng Lu, Beenish Bashir, Sajjad Hussain, Khalil Ahmad, Salahuddin Khan, Sajjad Haider, Zongxian Yang, Kersti Hermansson, Jun Li
Summary: This study systematically investigates the catalytic activity and stability of single noble metal atom catalysts supported on MXene materials for CO oxidation. The results show that CO oxidation mainly proceeds via the TER mechanism under mild reaction conditions. Ru1- and Ir1@Mo2CS2 exhibit high activity and catalytic stability.
CHINESE CHEMICAL LETTERS
(2023)
Article
Chemistry, Multidisciplinary
Ansheng Wang, Xilin Zhang, Shan Gao, Chunning Zhao, Siyu Kuang, Shanshan Lu, Juntao Niu, Geng Wang, Weifang Li, Da Chen, Haijun Zhang, Xiaomeng Zhou, Sheng Zhang, Bin Zhang, Weichao Wang
Summary: This study develops a reconstructed FeCoNiSx electrocatalyst for fast-charging Zn-air batteries. The electrocatalyst has a high density of efficient active sites, resulting in low oxygen evolution overpotentials. The fabricated Zn-air battery shows long lifetime and has potential for practical applications.
ADVANCED MATERIALS
(2022)
Article
Energy & Fuels
Xilin Zhang, Shihao Feng, Jiahang Yu, Runchuan Shi, Zhongjun Ma, Zongxian Yang, Lin Yang
Summary: In this study, the researchers demonstrated that the electronic structures and OER activity of confined Ni single atom catalyst (SAC) can be modulated by encapsulated Ni nanoparticles. The synergistic interaction between Ni SAC and Ni nanoparticles endowed the sample with satisfactory OER performance. Furthermore, the Ni-modified sample showed superior performance as an air-cathode catalyst for rechargeable zinc-air batteries.
Article
Physics, Applied
Yudong Pang, Zhansheng Lu, Shamraiz Hussain Talib, Xinyuan Li, Mingyang Wang, Xilin Zhang, Zongxian Yang, Ruqian Wu
Summary: This study investigates the effects of heteroatom doping and charge variation on the ability of MoS2 substrate to capture Na ions in sodium-ion batteries using first-principles calculations. The results show that Al- or Si-doped MoS2 can serve as good electrode materials with high theoretical capacity.
PHYSICAL REVIEW APPLIED
(2022)
Article
Chemistry, Physical
Xilin Zhang, Wenli Kang, Xiaodong Li, Qianqian Peng, Zongxian Yang, Weichao Wang
Summary: This study systematically explores the catalytic properties of a single Pt atom supported on PtS2, PtSe2, PtTe2 for CO oxidation. The results show that Pt1/PtTe2 exhibits the highest activity and provides an important reference for the design of SACs based on TMDs.
APPLIED SURFACE SCIENCE
(2023)
Article
Physics, Multidisciplinary
Qingfang Chang, Xilin Zhang, Zongxian Yang
Summary: This study systematically investigates the CO oxidation processes on a CuAu alloy monolayer supported on tungsten carbide, and compares it with pure metal monolayers using first-principles calculations. The introduction of Cu dopant in the Au monolayer enhances the adsorption of reactants, which lowers the energy barriers for the formation and dissociation of the intermediate OOCO. The rate determining step is identified as the oxidation of CO by an atomic O, with an energy barrier superior or comparable to reported CO oxidation catalysts. This work highlights the significance of alloy monolayers on tungsten carbides for the rational design of highly efficient catalysts.
Article
Physics, Multidisciplinary
Xinyuan Li, Yudong Pang, Mingyang Wang, Xilin Zhang, Zhansheng Lu, Zongxian Yang
Summary: Currently, MXenes have been recognized as a promising choice for Na-ion battery electrode materials due to their excellent energy storage and electrical conductivity. Among these, dual transition metal MXenes have gained attention as anode materials for Na-ion batteries because of their superior properties. In this study, we compared the performance of TiNbC-based dual transition metal MXenes and Nb2C-based single transition metal MXenes as anode materials for Na-ion batteries through density functional theory calculations. The results showed that TiNbC, TiNbCO2, Nb2C, and Nb2CO2 exhibited great potential as anode materials due to their low diffusion barrier and high Na capacity. Furthermore, TiNbC-based MXenes demonstrated better adsorption performance, diffusion rate, and theoretical storage of Na atoms compared to Nb2C-based MXenes, which was attributed to the synergistic effect between Ti and Nb. This discovery provides valuable insight for the development of high-performance MXenes-based anode materials for Na-ion batteries.
Article
Chemistry, Physical
Xilin Zhang, Shihao Feng, Runchuan Shi, Zhongjun Ma, Zongxian Yang
Summary: The catalytic activity of single metal atom can be enhanced by different coordination environments, mainly due to the modification of electronic structure by in-plane ligands. In this study, the multiple functions of axial oxygen ligand in improving the oxygen reduction activity were clarified using MoNO modified carbon as a representative example.
Article
Nanoscience & Nanotechnology
Qianqian Peng, Xilin Zhang, Zhi Geng, Zongxian Yang, Jubao Yang
Summary: In this study, the geometrical properties, electronic structure, and CO oxidation catalytic activity of Zn single atom catalyst on pristine and defective Ti2CT2 MXenes were investigated. Ti2CN2 was found to be an excellent substrate for stabilizing the Zn catalyst. The catalytic oxidation mechanism of CO on Zn-Ti2CN2 was studied, and the Eley-Rideal mechanism was identified as the most favorable pathway. The synergistic effects of the adsorbed Zn atom and the substrate were confirmed in regulating electron transfer and enhancing CO oxidation activity.
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES
(2023)
Article
Chemistry, Multidisciplinary
Zhenpu Shi, Juhong Xu, Yujiao Wang, Yudong Pang, Wanli Zhao, Hongyun Yue, Zongxian Yang, Shu-Ting Yang, Yanhong Yin
Summary: This study focuses on solving the problems of slow reaction kinetics and LiPSs shuttling in lithium-sulfur batteries by using a composite material of transition metal phosphides and carbon nanosheets as a sulfur host material. The introduction of CoP nanoparticles improves the reaction kinetics of LiPS conversion and increases the nucleation rate of Li2S, resulting in improved electrochemical performance of the composite as a sulfur host for lithium-sulfur batteries.
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2023)
Article
Chemistry, Physical
Mingyang Wang, Jianjun Mao, Yudong Pang, Xilin Zhang, Haiyan Wang, Zongxian Yang, Zhansheng Lu, Shuting Yang
Summary: This work reports on an effective strategy for enhancing the electrochemical performance of Li-S batteries by doping single atom Zn on the S-terminated Ti2C MXenes. The study elucidates the interactions between lithium polysulfides (LiPSs) and the Ti2-xZnxCS2 surface, as well as the delithiation process of Li2S on the Ti2-xZnxCS2 surface using spin-polarized density functional theory (DFT) calculations. The results demonstrate the importance of surface chemistry and electronic structure of MXenes in LiPSs' adsorption and catalysis capability, providing insights for the preparation and practical application of MXenes in Li-S batteries.
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
(2023)
Article
Chemistry, Inorganic & Nuclear
Zhenpu Shi, Yunqi Huang, Juhong Xu, Yudong Pang, Lan Wang, Wanli Zhao, Hongyun Yue, Zongxian Yang, Shuting Yang, Yanhong Yin
Summary: In this study, three-dimensional hierarchical porous carbon materials co-doped with B, N, and P and uniformly dispersed with CoP nanoparticles were synthesized and used as the coating material for the PE separator. Both experimental and theoretical calculations demonstrated that the adsorption capacity of the composite material for LiPS was significantly enhanced after introducing B atoms. As a result, LSBs assembled with the CoP@BNPC/PE separator exhibited excellent long-term stability and superior rate performance. This work further proves that a modified separator is an effective strategy for promoting the commercialization of LSBs.
DALTON TRANSACTIONS
(2023)
Article
Physics, Applied
Yudong Pang, Xilin Zhang, Mingyang Wang, Zhenpu Shi, Zongxian Yang, Zhansheng Lu, Ruqian Wu
Summary: This study introduces a descriptor (ε(α)) to efficiently identify high-performance electrode materials and reveals a robust linear relationship between the descriptor and adsorption energy. This finding serves as a practical guide for designing high-capacity battery materials and promotes future advancements in this field.
APPLIED PHYSICS LETTERS
(2023)
Article
Chemistry, Physical
Qi-Wen Chen, Ze-Qing Guo, Jian-Ping Zhou
Summary: Multifunctional continuous solid solutions NFMTO-x were successfully synthesized via a one-step hydrothermal method by controlling the ratio of Mg and Fe. The NFMTO-x materials exhibited enhanced visible light response, effective adsorption and photocatalytic degradation of organic pollutants, CO2 methanation capability, and easy recyclability due to their magnetic properties. This research provides a significant multifunctional material for water purification.
APPLIED SURFACE SCIENCE
(2024)
Review
Chemistry, Physical
George E. Stan, Maziar Montazerian, Adam Shearer, Bryan W. Stuart, Francesco Baino, John C. Mauro, Jose M. F. Ferreira
Summary: Bioactive glasses have the ability to form strong bonds with tissues and release therapeutic ions. However, their biomechanical compatibility limits their use in load-bearing applications. The use of magnetron sputtering technology to fabricate BG coatings shows promise in improving their efficacy and potential for application.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Zhaoxuan Wang, Zhicheng Yan, Zhigang Qi, Yu Feng, Qi Chen, Ziqi Song, Meng Huang, Peng Jia, Ki Buem Kim, Weimin Wang
Summary: The corrosion behavior of Fe-60 and Fe-83 ribbons in 0.6 M NaCl was studied. Fe-60 exhibited a local corrosion mode and formed a stable passivation film with higher corrosion resistance, while Fe-83 showed a combination of local and global corrosion modes and had lower corrosion resistance. Controlling the precipitation of nanocrystalline phases and increasing the POx content in the passivation film significantly improved the corrosion resistance of Fe-based glassy alloys.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Hao-Kai Peng, Sheng-Yen Zheng, Wei-Ning Kao, Ting-Chieh Lai, Kai-Sheun Lee, Yung- Hsien Wu
Summary: This study investigates the effects of high energy/fluence proton radiation on the performance of HfZrOx-based FeFETs memory with different Zr content. The results show that the characteristics of FeFETs are influenced by proton radiation, and the extent of the influence depends on the Zr content. FeFETs with 50% Zr content exhibit minimal changes in memory window and demonstrate good endurance and retention performance.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Zongyi Yue, Guangyi Wang, Zengguang Huang, Sihua Zhong
Summary: In this study, AZO and ITO films were successfully tuned as excellent passivation layers for c-Si surfaces, achieving effective minority carrier lifetime and outstanding optical properties through the optimization of annealing temperature and interfacial silicon oxide.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Martin Hruska, Jan Kejzlar, Jaroslav Otta, Premysl Fitl, Michal Novotny, Jakub Cizek, Oksana Melikhova, Matej Micusik, Peter Machata, Martin Vrnata
Summary: This paper presents a detailed study on the hydrogen sensing capabilities of highly nanoporous black gold films. The films exhibit fast response and recovery times at low temperatures. Different levels of nanoporosity were prepared and tested to investigate the sensing properties, and it was found that nanoporous black gold is suitable for hydrogen sensing. The sensitivity of the film depends on its nanoporosity.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yupu Wang, Gaofeng Teng, Chun To Yiu, Junyi Zhu
Summary: In the study of BM-SCO and HSCO thin films, it was found that H vacancies tend to prefer sites near the external surface or oxygen vacancy channels (OVCs), while H interstitials prefer sites of oxygen on a layer that contains six-fold coordinated Co. These findings not only enrich the understanding of complex surface phenomena of defect formation but also provide an explanation for the reversibility during phase transformation.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Jiafeng Lu, Linping Teng, Qinxiao Zhai, Chunhua Wang, Matthieu Lancry, Ye Dai, Xianglong Zeng
Summary: In this study, we achieved full control of fiber nanograting orientation by manipulating laser polarization, and tailored space variant fiber nanogratings, which expanded the diversity in fiber nanograting engineering.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yibo Liu, Yujie Tao, Yue Liu, Qi Sun, Qinrong Lin, Kexin Kang, Qinghua Zhang, Qingjie Sun
Summary: This study investigates the wettability of the Ti-Cu-Fe multi-metal system, specifically the wetting behaviors of CuSi3 droplets on TC4 and 304SS plates. The results show that the CO2 + Ar gas atmosphere significantly affects interfacial mass transfer, thus influencing the wettability of the systems.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Jimei Liu, Fei Wang, Rong Guo, Yuqi Liu, Mengyu Zhang, Jaka Sunarso, Dong Liu
Summary: This study developed Co/MXene composites with anti-corrosion properties by varying the cobalt content. These composites exhibited remarkable electromagnetic absorption performance and high resistance to corrosion under various corrosive conditions. The study also revealed the mechanism of electron transfer from cobalt to MXene and the electromagnetic dissipation behavior originated from polarization loss alone.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Moujie Huang, Yongsong Ma, Jingbo Yang, Lingyun Xu, Hangqi Yang, Miao Wang, Xin Ma, Xin Xia, Junhao Yang, Deli Wang, Chuang Peng
Summary: Strong metal-support interactions (SMSIs) are important for enhancing catalytic activities and stability in thermal catalysis. This study demonstrates a method to create SMSIs in electrocatalysis using carbon nanotubes and Ru nanoparticles, resulting in excellent catalytic activity and stability.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Ravi Trivedi, Brinti Mondal, Nandini Garg, Brahmananda Chakraborty
Summary: This study explores the potential of biphenylene as a nanocarrier for the delivery of the anticancer drug cisplatin. It is found that biphenylene offers physical stability, rapid release rate, solubility, and bio-compatibilities compared to other nanocarriers. The adsorption of cisplatin on the surface of biphenylene involves charge transfer from cisplatin to biphenylene. The drug is shown to be released at body temperature in an acidic environment. Biphenylene also exhibits excellent cytotoxicity activity and cellular uptake of the drug. Overall, biphenylene shows promise as a potential nanocarrier for cisplatin delivery.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Hyun Jeong, Hyeong Chan Suh, Ga Hyun Cho, Rafael Salas-Montiel, Hayoung Ko, Ki Kang Kim, Mun Seok Jeong
Summary: In this study, a potential platform to enhance Raman scattering and increase the number of observable Raman modes in monolayer transition metal dichalcogenides (TMDs) was proposed. The platform consisted of large-scale arrays of gold micropillars (MPs), which were able to enhance the Raman intensity of TMDs and make difficult-to-detect Raman modes observable. The platform showed great industrial advantages and wide applicability due to its low cost, simple process, large controllable area, and short process time.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yasir Abbas, Shafqat Ali, Sajjad Ali, Waqar Azeem, Zareen Zuhra, Haoliang Wang, Mohamed Bououdina, Zhenzhong Sun
Summary: In this study, FeOx@SPNO-C core-shell nanospheres as a catalyst for degradation of sulfamethoxazole (SMX) were successfully synthesized. The synergistic interaction between FeOx and SPNO-C, high carbon charge density, and the presence of C = O groups and N/Fe-Nx sites were found to be key factors for the enhanced degradation of SMX.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Qiaoting Yang, Yuxiao Gong, Yan Qian, Zhou-Qing Xiao, Serge Cosnier, Xue-Ji Zhang, Robert S. Marks, Dan Shan
Summary: This study proposes a hierarchical confinement strategy to design Prussian blue nanoparticles (PB NPs) with satisfactory electrocatalytic ability and stability. The catalytic synthesis of PB NPs is achieved through a hydrothermal process, and the as-prepared PB@NH2MIL exhibits efficient electronic transmission and enhanced electrocatalytic properties.
APPLIED SURFACE SCIENCE
(2024)