4.7 Article

Structure origin of a transition of classic-to-avalanche nucleation in Zr-Cu-Al bulk metallic glasses

期刊

ACTA MATERIALIA
卷 149, 期 -, 页码 108-118

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.actamat.2018.02.028

关键词

Bulk metallic glasses; Glass-forming ability; Crystallization kinetics; Neutron diffraction

资金

  1. Research Grants Council of Hong Kong Special Administrative Region (CityU) [11216215]
  2. National Natural Science Foundation of China [51571170]
  3. Croucher Foundation (CityU) [9500020]
  4. National Science Foundation of China [51501090, 51520105001]
  5. Natural Science Foundation of Jiangsu Province [BK20171425]
  6. Fundamental Research Funds for the Central Universities [30915015103]
  7. Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC05-00OR22725]
  8. Oak Ridge National Laboratory

向作者/读者索取更多资源

Crystallization kinetics of a series of Zr-Cu-Al bulk metallic glasses with different glass-forming abilities were systematically investigated using differential scanning calorimetry, time-resolved neutron diffraction, and high-resolution transmission electron microscopy. Experimental results revealed a transition of classic-to-avalanche types of nucleation for the Zr-Cu-Al glass alloys upon isothermal annealing. The classic mode is characterized by a continuous nucleation and growth of Zr2Cu-type crystals. The avalanche mode features an abrupt formation of massive Cu10Zr7-type precipitates with a complex, low-symmetry crystalline structure. Calorimetric measurements identified an anomalous exothermic peak prior to crystallization for metallic glasses with the Cu10Zr7-type crystalline phase. The formation of a metastable amorphous/semi-crystalline phase was observed using the electron microscopy prior to crystallization for glasses with an anomalous exothermic event. Our results indicate that the formation of a metastable phase might lower the free energy barrier of the crystallization and trigger an avalanche type of nucleation. Neutron diffraction pair distribution function analysis suggests that the easy connection of short-range clusters at the medium-range length scale would favor the avalanche nucleation. (C) 2018 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.7
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Computer Science, Artificial Intelligence

Attention Enhanced Reinforcement Learning for Multi agent Cooperation

Zhiqiang Pu, Huimu Wang, Zhen Liu, Jianqiang Yi, Shiguang Wu

Summary: In this article, a novel method called AERL is proposed to address complex interaction and communication issues in multi agent cooperation. The method utilizes attention mechanism and parameter sharing to achieve effective and robust performance, as demonstrated in simulation experiments in three representative scenarios.

IEEE TRANSACTIONS ON NEURAL NETWORKS AND LEARNING SYSTEMS (2023)

Article Public, Environmental & Occupational Health

The 100 most-cited articles on bibliotherapy: a bibliometric analysis

Zheng Xu, Ru Liu, Liping Guo, Ziyi Gao, Zicheng Gao, Xiaowei Liu, Jieyun Li, Bin Li, Kehu Yang

Summary: This scientometric investigation provides a comprehensive analysis of the development and emerging research trends in bibliotherapy. The study identifies the leading countries and institutions in the field and highlights the hot topics of research, such as depression and anxiety. The findings of this study serve as a valuable reference for researchers in the field of bibliotherapy.

PSYCHOLOGY HEALTH & MEDICINE (2023)

Article Automation & Control Systems

Enhanced fractional order sliding mode control for a class of fractional order uncertain systems with multiple mismatched disturbances

Weijia Zheng, YangQuan Chen, Xiaohong Wang, Yong Chen, Meijin Lin

Summary: In this paper, an enhanced fractional order sliding mode control (FOSMC) method is proposed to improve the control performance of fractional order uncertain systems with multiple mis-matched disturbances. The multiple disturbances and uncertainties are estimated by finite-time disturbance observers and a fractional order extended state observer. A fractional order switching law is designed for fast convergence of system states. The proposed method incorporates feedforward compensation, the fractional order switching law, and an auxiliary state for input saturation. Numerical examples and a motor speed control problem are used to demonstrate the effectiveness of the proposed method through performance comparisons with existing control methods.

ISA TRANSACTIONS (2023)

Article Engineering, Electrical & Electronic

Analysis of Electronic Characteristics of Plasma-Enhanced Indium Zinc Oxide Thin Film Transistors

Fei Shan, Suchang Yoo, Jae-Yun Lee, Han-Lin Zhao, Xiao-Lin Wang, Seong Gon Choi, Heung Gyoon Ryu, Yong Jin Jeong, Sung-Jin Kim

Summary: In this paper, a multi-stacked IZO TFT with exceptional electronic characteristics is prepared, and the plasma treatment is used to improve the performance of the device and optimize the crystal structure and surface smoothness.

JOURNAL OF ELECTRICAL ENGINEERING & TECHNOLOGY (2023)

Article Obstetrics & Gynecology

Comparative Proteomic and Phospho-proteomic Analysis of Mouse Placentas Generated via In Vivo and In Vitro Fertilization

Jie Dong, Qian Xu, Shuqiang Chen, Hui Lei, Jingjing Wang, Song Yan, Chenxi Qian, Xiaohong Wang

Summary: "Offspring conceived by assisted reproductive technologies (ART) have an increased risk of gestational complications, which are related to placental dysfunction. This study used proteomics and phospho-proteomics to investigate the underlying mechanisms responsible for the changes in ART placentas. The findings suggest that ART leads to altered cell junctions, renin-angiotensin system, amino acid transport, and increased mTOR signaling in mouse placentas."

REPRODUCTIVE SCIENCES (2023)

Article Biotechnology & Applied Microbiology

Synergy of antioxidant and M2 polarization in polyphenol-modified konjac glucomannan dressing for remodeling wound healing microenvironment

Huiyang Li, Xiaoyu Liang, Youlu Chen, Kaijing Liu, Xue Fu, Chuangnian Zhang, Xiaoli Wang, Jing Yang

Summary: In this study, a wound dressing composed of konjac glucomannan and gallic acid was developed, which could accelerate wound healing by promoting macrophage polarization and reducing reactive oxygen species levels. In vivo experiments showed that it had excellent anti-inflammatory properties.

BIOENGINEERING & TRANSLATIONAL MEDICINE (2023)

Article Cardiac & Cardiovascular Systems

PTX3 from vascular endothelial cells contributes to trastuzumab-induced cardiac complications

Zhifei Xu, Zizheng Gao, Huangxi Fu, Yan Zeng, Ying Jin, Bo Xu, Yuanteng Zhang, Zezheng Pan, Xueqin Chen, Xiaochen Zhang, Xiaohong Wang, Hao Yan, Xiaochun Yang, Bo Yang, Qiaojun He, Peihua Luo

Summary: This study identified a distinct mechanism of trastuzumab-induced cardiac complications through the promotion of PTX3 excretion in vascular endothelial cells, leading to impaired contractility of cardiomyocytes. Inhibition of the EGFR/STAT3 signaling pathway reduced the release of PTX3, thereby blocking the cardiac side effects caused by trastuzumab.

CARDIOVASCULAR RESEARCH (2023)

Review Clinical Neurology

A Meta-analysis of the Clinical Efficacy of the Head-of-Bed Elevation for Patients With Acquired Brain Injury

Ying Che, Tingting Lu, Tianming Wang, Hairong Zhao, Xulin Song, Qing Zhan, Chengzu Zhang, Haibang Pan, Kehu Yang, Bo Wang

Summary: This study evaluated the effects of head-of-bed elevation on patients with acquired brain injury (ABI). The results showed that elevating the head of the bed by 30 degrees can significantly reduce intracranial pressure (ICP), but did not have statistical differences on cerebral perfusion pressure (CPP) and disability at 90 days. Therefore, head-of-bed elevation of 30 degrees may be an effective noninvasive nursing practice for the prognosis and rehabilitation of ABI patients.

JOURNAL OF NEUROSCIENCE NURSING (2023)

Review Sport Sciences

Pilates and multiple health outcomes: An umbrella review

Meng Xu, Chen Tian, Yong Wang, Shanshan Liang, Yiyun Wang, Xiuxia Li, Kehu Yang

Summary: This study conducted an umbrella review to summarize the evidence of associations between Pilates and multiple health outcomes, and evaluated the strength and validity of these associations. It found that Pilates can reduce body mass index and body fat percentage, relieve pain and disability, and improve sleep quality and balance. However, the certainty of the evidence was mostly low, and further high quality randomized controlled trials are needed to support these promising findings.

JOURNAL OF SCIENCE AND MEDICINE IN SPORT (2023)

Review Integrative & Complementary Medicine

Adverse effects associated with acupuncture therapies: An evidence mapping from 535 systematic reviews

Meng Xu, Chaoqun Yang, Tao Nian, Chen Tian, Liying Zhou, Yanan Wu, Yanfei Li, Xinxin Deng, Xiuxia Li, Kehu Yang

Summary: This study examines the adverse effects of acupuncture and finds that there are various types of adverse reactions, but the symptoms are mild. However, most of the included studies have low quality, indicating a need for further randomized controlled trials and systematic reviews to comprehensively analyze acupuncture-related adverse events.

CHINESE MEDICINE (2023)

Review Emergency Medicine

Effectiveness of intraoperative peritoneal lavage with saline in patient with intra-abdominal infections: a systematic review and meta-analysis

Qi Zhou, Wenbo Meng, Yanhan Ren, Qinyuan Li, Marja A. Boermeester, Peter Muli Nthumba, Jennifer Rickard, Bobo Zheng, Hui Liu, Qianling Shi, Siya Zhao, Zijun Wang, Xiao Liu, Zhengxiu Luo, Kehu Yang, Yaolong Chen, Robert G. Sawyer

Summary: This study reviewed the effectiveness of intraoperative peritoneal lavage (IOPL) with saline in patients with intra-abdominal infections (IAIs). The findings suggest that IOPL with saline does not significantly reduce the risk of mortality, intra-abdominal abscess, incisional surgical site infection, postoperative complication, reoperation, and readmission when compared to non-IOPL. Therefore, routine use of IOPL with saline in patients with IAIs is not supported.

WORLD JOURNAL OF EMERGENCY SURGERY (2023)

Article Engineering, Environmental

ILTox: A Curated Toxicity Database for Machine Learning and Design of Environmentally Friendly Ionic Liquids

Jiachen Yan, Guohong Liu, Hanle Chen, Song Hu, Xiaohong Wang, Bing Yan, Xiliang Yan

Summary: A comprehensive online database on the toxicity of ionic liquids (ILs) has been developed to aid in the design of environmentally friendly ILs using machine learning. The ILTox database contains manually curated data, including 1183 ILs and over 6700 pieces of toxicity data across different organisms. Machine learning models have been constructed using this database to analyze the relationship between IL structures and toxicities. The database has been used for virtual screening of desired IL properties from a large pool of ILs and has proven to be a valuable resource in understanding IL toxicity.

ENVIRONMENTAL SCIENCE & TECHNOLOGY LETTERS (2023)

Article Chemistry, Physical

An anomalous structure disordering in Zr-Cu-Ag supercooled glass-forming liquids

Yu Lou, Sinan Liu, Jiacheng Ge, Huiqiang Ying, Shu Fu, Wentao Zhang, Weixia Dong, Zhenduo Wu, Xun-Li Wang, Elliot P. Gilbert, Yang Ren, Si Lan

Summary: An anomalous ordering-to-disordering transition in a Zr-Cu-Ag supercooled glass-forming liquid was observed using in situ high-energy x-ray diffraction. Heating the supercooled liquid showed a structural crossover at Tc = 716 K, as indicated by changes in the statistical characteristics of the first sharp diffraction peak. Annealing the supercooled liquid near Tc initially led to relaxation towards a denser and more ordered state. Eventually, the liquid became disordered at a medium-range scale, with a slow densification process.

INTERMETALLICS (2023)

Article Chemistry, Multidisciplinary

In situ growth of TiO2/Ti3C2 MXene Schottky heterojunction as a highly sensitive photoelectrochemical biosensor for DNA detection

Caiyan Lai, Bingdong Yan, Run Yuan, Delun Chen, Xiaohong Wang, Mingyu Wang, Heyu He, Jinchun Tu

Summary: In this study, a heterojunction composed of a TiO2 nanosheet and layered Ti3C2 was synthesized. The TiO2/Ti3C2 composites exhibited increased surface area and extended light absorption range, leading to prolonged lifetime of photogenerated carriers. A photoelectrochemical DNA biosensor based on the TiO2/Ti3C2 heterostructure was constructed and comprehensively studied. The sensor displayed stability and sensitivity for DNA detection in the range of 10 nM-10 fM, with a lower detection limit of 6 fM. It provided potential for early diagnosis of various diseases by detecting target DNA.

RSC ADVANCES (2023)

Article Engineering, Environmental

Preparation of activated biochar with adjustable pore structure by hydrothermal carbonization for efficient adsorption of VOCs and its practical application prospects

Fan Yao, Guangzheng Ye, Weixiao Peng, Guangyi Zhao, Xiaohong Wang, Yuqin Wang, Wenfu Zhu, Yujun Jiao, Haomin Huang, Daiqi Ye

Summary: This study investigates the hydrothermal carbonization (HTC) of glucose and precisely determines the pore structure of the obtained hydrochar by controlling the main factors of the hydrothermal process. The results provide guidance and an effective reference for the pore size adjustment of porous-activated biochar developed for the adsorption of pollutants.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2023)

Article Materials Science, Multidisciplinary

Transmission electron microscopy of the rapid solidification microstructure evolution and solidification interface velocity determination in hypereutectic Al-20at.%Cu after laser melting

Y. Liu, K. Zweiacker, C. Liu, J. T. McKeown, J. M. K. Wiezorek

Summary: The evolution of rapid solidification microstructure and solidification interface velocity of hypereutectic Al-20at.%Cu alloy after laser melting has been studied experimentally. It was found that the formation of microstructure was dominated by eutectic, alpha-cell, and banded morphology grains, and the growth modes changed with increasing interface velocity.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Mechanisms for high creep resistance in alumina forming austenitic (AFA) alloys

Bharat Gwalani, Julian Escobar, Miao Song, Jonova Thomas, Joshua Silverstein, Andrew Chihpin Chuang, Dileep Singh, Michael P. Brady, Yukinori Yamamoto, Thomas R. Watkins, Arun Devaraj

Summary: Castable alumina forming austenitic alloys exhibit superior creep life and oxidation resistance at high temperatures. This study reveals the mechanism behind the enhanced creep performance of these alloys by suppressing primary carbide formation and offers a promising alloy design strategy for high-temperature applications.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Achieving atomically flat copper surface: Formation of mono-atomic steps and associated strain energy mechanisms

Jian Song, Qi Zhang, Songsong Yao, Kunming Yang, Houyu Ma, Jiamiao Ni, Boan Zhong, Yue Liu, Jian Wang, Tongxiang Fan

Summary: Recent studies have shown that achieving an atomically flat surface for metals can greatly improve their oxidation resistance and enhance their electronic-optical applications. Researchers have explored the use of graphene as a covering layer to achieve atomically flat surfaces. They found that high-temperature deposited graphene on copper surfaces formed mono-atomic steps, while annealed copper and transferred graphene on copper interfaces formed multi-atomic steps.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Modeling and measurements of creep deformation in laser-melted Al-Ti-Zr alloys with bimodal grain size

Jennifer A. Glerum, Jon-Erik Mogonye, David C. Dunand

Summary: Elemental powders of Al, Ti, Sc, and Zr are blended and processed via laser powder-bed fusion to create binary and ternary alloys. The microstructural analysis and mechanical testing show that the addition of Ti results in the formation of primary precipitates, while the addition of Sc and Zr leads to the formation of fine grain bands. The Al-0.25Ti-0.25Zr alloy exhibits comparable strain rates to Al-0.5Zr at low stresses, but significantly higher strain rates at higher stresses during compressive creep testing. Finite element modeling suggests that the connectivity of coarse and fine grain regions is a critical factor affecting the creep resistance of the alloys.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Characterizing stable nanocrystalline Cu-Ta behavior and failure dynamics under extremes of strain rate, strain, temperature and pressure by modified dynamic tensile extrusion

P. Jannotti, B. C. Hornbuckle, J. T. Lloyd, N. Lorenzo, M. Aniska, T. L. Luckenbaugh, A. J. Roberts, A. Giri, K. A. Darling

Summary: This work characterizes the thermo-mechanical behavior of bulk nanocrystalline Cu-Ta alloys under extreme conditions. The experiments reveal that the alloys exhibit unique mechanical properties, behaving differently from conventional nanocrystalline Cu. They do not undergo grain coarsening during extrusion and exhibit behavior similar to coarse-grained Cu.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Phase-dependent microstructure modification leads to high thermoelectric performance in n-type layered SnSe2

Yiqing Wei, Jingwei Li, Daliang Zhang, Bin Zhang, Zizhen Zhou, Guang Han, Guoyu Wang, Carmelo Prestipino, Pierric Lemoine, Emmanuel Guilmeau, Xu Lu, Xiaoyuan Zhou

Summary: This study proposes a new strategy to modify microstructure by phase regulation, which can simultaneously enhance carrier mobility and reduce lattice thermal conductivity. The addition of Cu in layered SnSe2 induces a phase transition that leads to increased grain size and reduced stacking fault density, resulting in improved carrier mobility and lower lattice thermal conductivity.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Selective oxidation and nickel enrichment hinders the repassivation kinetics of multi-principal element alloy surfaces

Jia Chen, Zhengyu Zhang, Eitan Hershkovitz, Jonathan Poplawsky, Raja Shekar Bhupal Dandu, Chang-Yu Hung, Wenbo Wang, Yi Yao, Lin Li, Hongliang Xin, Honggyu Kim, Wenjun Cai

Summary: In this study, the structural origin of the pH-dependent repassivation mechanisms in multi-principal element alloys (MPEA) was investigated using surface characterization and computational simulations. It was found that selective oxidation in acidic to neutral solutions leads to enhanced nickel enrichment on the surface, resulting in reduced repassivation capability and corrosion resistance.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Rate-dependent transition of dislocation mechanisms in a magnesium alloy

X. Y. Xu, C. P. Huang, H. Y. Wang, Y. Z. Li, M. X. Huang

Summary: The limited slip systems of magnesium (Mg) and its alloys hinder their wide applications. By conducting tensile straining experiments, researchers discovered a rate-dependent transition in the dislocation mechanisms of Mg alloys. At high strain rates, glissile dislocations dominate, while easy-glide dislocations dominate at low strain rates. Abundant glissile dislocations do not necessarily improve ductility.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

The effect of temperature on detwinning and mechanical properties of face-centered cubic deformation twins

M. S. Szczerba, M. J. Szczerba

Summary: Inverse temperature dependences of the detwinning stress were observed in face-centered cubic deformation twins in Cu-8at.%Al alloy. The detwinning stress increased with temperature when the pi detwinning mode was involved, but decreased when the pi/3 mode was involved. The dual effect of temperature on the detwinning stress was due to the reduction of internal stresses pre-existing within the deformation twins. The complete reduction of internal stresses at about 530 degrees C led to the equivalence of the critical stresses of different detwinning modes and a decrease in the yield stress anisotropy of the twin/matrix structure.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Nature of the electric double layer to modulate the electrochemical behaviors of Fe2O3 electrode

Taowen Dong, Tingting Qin, Wei Zhang, Yaowen Zhang, Zhuoran Feng, Yuxiang Gao, Zhongyu Pan, Zixiang Xia, Yan Wang, Chunming Yang, Peng Wang, Weitao Zheng

Summary: The interaction between the electrode and the electric double layer (EDL) significantly influences the energy storage mechanism. By studying the popular alpha-Fe2O3 electrode and the EDL interaction, we find that the energy storage mechanism of the electrode can be controlled by modulating the EDL.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Grain scale bursts of plasticity in Mg-4Zn via high energy X-rays: Towards twin observation in real-time

Matthew R. Barnett, Jun Wang, Sitarama R. Kada, Alban de Vaucorbeil, Andrew Stevenson, Marc Fivel, Peter A. Lynch

Summary: The elastic-plastic transition in magnesium alloy Mg-4.5Zn exhibits bursts of deformation, which are characterized by sudden changes in grain orientation. These bursts occur in a coordinated manner among nearby grains, with the highest burst rate observed at the onset of full plasticity. The most significant burst events are associated with twinning, supported by the observation of twinned structures using electron microscopy. The bursts are often preceded and followed by a stasis in peak movement, indicating a certain "birth size" for twins upon formation and subsequent growth at a later stage.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Atomistic simulations and machine learning of solute grain boundary segregation in Mg alloys at finite temperatures

Vaidehi Menon, Sambit Das, Vikram Gavini, Liang Qi

Summary: Understanding solute segregation thermodynamics is crucial for investigating grain boundary properties. The spectral approach and thermodynamic integration methods can be used to predict solute segregation behavior at grain boundaries and compare with experimental observations, thus aiding in alloy design and performance control.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Integrating abnormal thermal expansion and ultralow thermal conductivity into (Cd,Ni)2Re2O7 via synergy of local structure distortion and soft acoustic phonons

Feiyu Qin, Lei Hu, Yingcai Zhu, Yuki Sakai, Shogo Kawaguchi, Akihiko Machida, Tetsu Watanuki, Yue-Wen Fang, Jun Sun, Xiangdong Ding, Masaki Azuma

Summary: This study reports on the negative and zero thermal expansion properties of Cd2Re2O7 and Cd1.95Ni0.05Re2O7 materials, along with their ultra-low thermal conductivity. Through investigations of their structures and phonon calculations, the synergistic effect of local structure distortion and soft phonons is revealed as the key to achieving these distinctive properties.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

Semi-automatic miniature specimen testing method to characterize the plasticity and fracture properties of metals

Thomas Beerli, Christian C. Roth, Dirk Mohr

Summary: A novel testing system for miniature specimens is designed to characterize the plastic response of materials for which conventional full-size specimens cannot be extracted. The system has an automated operation process, which reduces the damage to specimens caused by manual handling and improves the stability of the test results. The experiments show that the miniature specimens extracted from stainless steel and aluminum have high reproducibility, and the results are consistent with those of conventional-sized specimens. A correction procedure is provided to consider the influence of surface roughness and heat-affected zone caused by wire EDM.

ACTA MATERIALIA (2024)

Article Materials Science, Multidisciplinary

The effect of microstructure and film composition on the mechanical properties of linear antenna CVD diamond thin films

Rani Mary Joy, Paulius Pobedinskas, Nina Baule, Shengyuan Bai, Daen Jannis, Nicolas Gauquelin, Marie-Amandine Pinault-Thaury, Francois Jomard, Kamatchi Jothiramalingam Sankaran, Rozita Rouzbahani, Fernando Lloret, Derese Desta, Jan D'Haen, Johan Verbeeck, Michael Frank Becker, Ken Haenen

Summary: This study investigates the influence of film microstructure and composition on the Young's modulus and residual stress in nanocrystalline diamond thin films. The results provide insights into the mechanical properties and intrinsic stress sources of these films, and demonstrate the potential for producing high-quality nanocrystalline diamond films under certain conditions.

ACTA MATERIALIA (2024)