期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 5, 期 18, 页码 8416-8422出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7ta00539c
关键词
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资金
- Shenzhen Jiawei Photovoltaic Lighting Co. Ltd
- Tsinghua University Initiative Scientific Research Program [20161080165]
High efficiency perovskite solar cells can be made through the Lewis adduct approach. The interaction between PbI2 and the Lewis base is a key factor to make high quality perovskite films. Here, we combine a two-step method with the Lewis adduct approach to fabricate high quality organometallic perovskite films by tuning the strength of the Pb-O bond in Lewis acid-base adducts via adding different Lewis base additives. By optimizing the strength of the Pb-O bond, smooth CH3NH3PbI3 films with large perovskite grains are prepared. The high quality CH3NH3PbI3 films lead to a low recombination rate, long carrier life time and highly efficient charge transfer process. As a result, the power conversion efficiency of the best perovskite solar cell increases from 12.79% to 17.26%.
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