期刊
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
卷 2015, 期 9, 页码 1910-1914出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201403479
关键词
Ylides; Alkylation; Cross-coupling; Regioselectivity; Radicals
资金
- National Nature Science Foundation of China (NSFC) [21272069, 20672035]
- Fundamental Research Funds for the Central Universities
- Key Laboratory of Organofluorine Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences
A catalytic amount of benzoyl peroxide (BPO)-initiated cross-dehydrogenative coupling reaction of N-iminopyridine ylides with simple alkanes and alcohols leads to the corresponding 2-alkylpyridines with high regioselectivity in moderate to good yields without an additional reduction step to remove the activated group.
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