期刊
ACS CATALYSIS
卷 7, 期 9, 页码 6342-6346出版社
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.7b02356
关键词
C-H activation; S,O-ligand; olefination; palladium; arenes
资金
- NWO though a VIDI [723.013.006]
- Vicerrectorate of Research, Development and Innovation at the University of Alicante (Spain)
Pd(II)-catalyzed C-H functionalization of non directed arenes has been realized using an inexpensive and easily accessible type of bidentate S,O-ligand. The catalytic system shows high efficiency in the C-H olefination reaction of electron-rich and electron-poor arenes. This methodology is operationally simple, scalable, and can be used in late-stage functionalization of complex molecules. The broad applicability of this catalyst has been showcased in other transformations such as Pd(II)-catalyzed C-H acetoxylation and allylation reactions.
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