期刊
NATURE COMMUNICATIONS
卷 8, 期 -, 页码 -出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/s41467-017-00777-0
关键词
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资金
- DOE [DE-FG02-03ER46066]
- U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division
- Department of Energy [DE-FG02-04ER46111]
- Xunta de Galicia [EM2013/037]
- MINECO [MAT2013-44673-R]
- Ramon y Cajal Program [RyC2011-09024]
- Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]
Layered nickelates have the potential for exotic physics similar to high T-C superconducting cuprates as they have similar crystal structures and these transition metals are neighbors in the periodic table. Here we present an angle-resolved photoemission spectroscopy (ARPES) study of the trilayer nickelate La4Ni3O10 revealing its electronic structure and correlations, finding strong resemblances to the cuprates as well as a few key differences. We find a large hole Fermi surface that closely resembles the Fermi surface of optimally hole- doped cuprates, including its d(x)(-)(2) (2)(y) orbital character, hole filling level, and strength of electronic correlations. However, in contrast to cuprates, La4Ni3O10 has no pseudogap in the d(x)(-y)(2)(2) band, while it has an extra band of principally d(3z)(-r)(2)(2) orbital character, which presents a low temperature energy gap. These aspects drive the nickelate physics, with the differences from the cuprate electronic structure potentially shedding light on the origin of superconductivity in the cuprates.
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