4.8 Article

Extremely Large Magnetoresistance in a Topological Semimetal Candidate Pyrite PtBi2

期刊

PHYSICAL REVIEW LETTERS
卷 118, 期 25, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.118.256601

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资金

  1. Natural Science Foundation of China [11574320, 11374302, 11204312, 11474289, U1432251, 11674311, 11474030]
  2. National Key Research and Development Program of China [2016YFA0401003]
  3. 100 Talents Program of Chinese Academy of Sciences (CAS)

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While pyrite-type PtBi2 with a face-centered cubic structure has been predicted to be a three-dimensional (3D) Dirac semimetal, experimental study of its physical properties remains absent. Here we report the angular-dependent magnetoresistance measurements of a PtBi2 single crystal under high magnetic fields. We observed extremely large unsaturated magnetoresistance (XMR) up to (11.2x10(6)) % at T = 1.8 K in a magnetic field of 33 T, which is comparable to the previously reported Dirac materials, such as WTe2, LaSb, and NbP. The crystals exhibit an ultrahigh mobility and significant Shubnikov-de Hass quantum oscillations with a nontrivial Berry phase. The analysis of Hall resistivity indicates that the XMR can be ascribed to the nearly compensated electron and hole. Our experimental results associated with the ab initio calculations suggest that pyrite PtBi2 is a topological semimetal candidate that might provide a platform for exploring topological materials with XMR in noble metal alloys.

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