期刊
ORGANIC LETTERS
卷 19, 期 9, 页码 2206-2209出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b00463
关键词
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资金
- Ministry of Science and Technology of China [2013CB834804, 2013CB834505, 2014CB239402]
- National Natural Science Foundation of China [21390404, 91427303, 21402217]
- Strategic Priority Research Program of Chinese Academy of Sciences [XDB17030400]
- Technical Institute of Physics and Chemistry, CAS
Aryl ethers can be constructed from the direct coupling between the benzene C-H bond and the alcohol O-H bond with the evolution of hydrogen via the synergistic merger of photocatalysis and cobalt catalysis. Utilizing the dual catalyst system consisting of 3-cyano-l-methylquinolinum photocatalyst and cobaloxime, intermolecular etherification of arenes with various alcohols and intramolecular alkoxylation of 3-phenylpropanols with formation of chromanes are accomplished. These reactions proceed at remarkably mild conditions, and the sole byproduct is equivalent hydrogen gas.
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