期刊
ORGANIC LETTERS
卷 19, 期 6, 页码 1470-1473出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b00464
关键词
-
资金
- JSPS KAKENHI [JP16H06351, JP16H01137]
- Grants-in-Aid for Scientific Research [16H06351] Funding Source: KAKEN
The first enantioselective total syntheses of engelharquinone (2) and its epoxide 3 have been achieved. The key steps include (1) catalytic asymmetric 1,4-addition of a naphthylboronic acid derivative to a masked naphthoquinone derivative by using a chiral Rh-complex and (2) thiolate-promoted stereospecific construction of the bicyclo[3.2.1]octadienone scaffold.
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