期刊
ORGANIC LETTERS
卷 19, 期 22, 页码 6240-6243出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b03204
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资金
- NSFC [21522202, 21502017, 21273140]
- OIT program of Shanxi
An electron-withdrawing-group-generable radical-induced enamination of vinyl azides is reported, which results in a variety of beta-functionalized N-unprotected enamines in a stereoselective manner. A plausible mechanism involving an unusual 1,3-H transfer of in situ generated iminyl radical intermediate was proposed on the basis of experimental results and DFT calculations.
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