期刊
ORGANIC LETTERS
卷 19, 期 11, 页码 2913-2916出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b01149
关键词
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资金
- ACT-C from Japan Science and Technology Agency (Japan) [JPMJCR1122YR]
- JSPS Research Fellowship for Young Scientists [15J07947]
- Grants-in-Aid for Scientific Research [15J07947] Funding Source: KAKEN
It has been established that a cationic rhodium(I)/(R)-MeO-BIPHEP complex catalyzes the asymmetric [2 + 2 + 2] cyclization of 1,6-enynes with aliphatic and aromatic alkenes to produce chiral cyclic dienes through beta-hydride elimination from rhodacycle intermediates. Thus, obtained chiral cyclic dienes could be converted to chiral spirocompounds without racemization.
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