期刊
MATERIALS CHEMISTRY AND PHYSICS
卷 198, 期 -, 页码 186-192出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.matchemphys.2017.05.020
关键词
Nanocomposites; Carbon nano-onions; Adsorption; Bisphenol A
资金
- National Natural Science Foundation of China [21275131, 21607135]
- Zhejiang Environmental Protection Bureau [2013A025]
- Key Discipline of Chemistry in Zhejiang Provincial Colleges (Zhejiang Normal University) [ZJHX201522]
- Key Laboratory of the Ministry of Education for Advanced Catalytic Materials (Zhejiang Normal University) [ZJHX201522]
In this work, a scalable and cost-effective approach was developed for the synthesis of magnetic carbon nano-onions (MCNOs) by using iron (III) acetylacetonate modified candle as the raw materials. The candle soot was collected from the burning candle and then subjected to calcination at 800 degrees C under N-2 atmosphere. The obtained MCNOs were further applied as adsorbent for the removal of bisphenol A (BPA) from aqueous solutions. Adsorption of BPA onto the MCNOs was investigated with the influence of initial concentration of BPA, solution pH, and adsorption time. The results demonstrated the adsorption of BPA onto the MCNOs was almost not affected by pH in the range from 5-9. The adsorption isothermal and kinetic's data were better fitted by Langmuir isotherm and pseudo-second-order kinetic model, respectively. Moreover, the MCNOs are easily recycled by using and external magnet and regenerated by simply methanol washing. The results present here not only provide a novel synthetic approach toward low-cost nanocarbons but also revealed the great application potential of the MCNOs for the removal of endocrine disrupting compounds from aqueous solution. (C) 2017 Elsevier B.V. All rights reserved.
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