期刊
MACROMOLECULAR MATERIALS AND ENGINEERING
卷 302, 期 10, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/mame.201700102
关键词
biomimetic fiber; dry spinning; microfluidic chip; silk fibroin; spindle-knots
资金
- National Natural Science Foundation of China [21674018, 21274018]
- National Key Research and Development Program of China [2016YFA0201702/2016YFA0201700]
- Shuguang Program - Shanghai Education Development Foundation and Shanghai Municipal Education Commission [15SG30]
- DHU Distinguished Young Professor Program [A201302]
- Fundamental Research Funds for the Central Universities
Spider and silkworm produce diverse silk fibers from spinning dopes through smart spinnerets. Spider's capture silk is composed of core thread and periodic spindle-knots, while silkworm silk consists of fibroin core and sericin outer layer. To mimic the morphologies of natural heterostructured silks, artificial fibers are dry-spun using a multichannel microfluidic chip, served with a highly viscous core solution of regenerated silk fibroin and low viscosity sheath solution of sericin. Silk fibers with core-sheath, groove, and spindle-knot structures are obtained by controlling the flow rates and viscosities of the two microfluids depending on the laminar flow, Kelvin-Helmholtz instability, or Plateau-Rayleigh instability.
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