期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 139, 期 44, 页码 15644-15647出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.7b10130
关键词
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资金
- NSERC-DG
- ERA
- CFI
- Brock University (Chancellor's Chair for Research Excellence)
- Ministerio de Economia y Competitividad [CTQ2015-63614-P]
The first {Mn-31} cluster (1) has been prepared from carboxylate ions and the chelating/bridging ligand alpha-methyl-2-pyridine-methanol. Compound 1 possesses a unique nanosized structural topology with one of the largest energy barriers reported to-date for high-nuclearity 3d-metal clusters. Single-crystal magnetic hysteresis studies reveal the presence of hysteresis loops below 5 K, one of the highest temperatures below which molecular hysteresis has been observed for 3d-based SMMs.
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