期刊
JOURNAL OF ELECTROANALYTICAL CHEMISTRY
卷 804, 期 -, 页码 179-184出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.jelechem.2017.09.062
关键词
Nitrogen doping; Capacitive deionization; Cocoon; Electrosorption
资金
- National Natural Science Foundation of China [21276087]
Capacitive deionization (CDI) has been attracted great mterest as an emerging desalination technology and the electrode materials play a critical role on improving CDI performance. In this work, nitrogen-enriched activated carbon fibers (AN-CFs) were prepared from the natural based silk cocoon through simple carbonization and CO(2)activation. Their electrochemical and electrosorption behaviors were studied in NaCl solution. The results show that AN-CFs exhibit a fibri form porous structure with rich nitrogen element and CO(2)activation enhances their specific surface area. Compared with unactivated nitrogen-enriched carbon fibers (196.05 F g (-1) at 1 mV s(-1)12.02 mg g(-1) in 1000 mg l(-1) NaCl solution), AN-CFs exhibit more excellent capacitive (236.03 F g (-x)) and CDI (16.56mg g(-1)) performances, showing that CO2 activation is proved to be an effective method to improve electrochemical and electrosorption performances and the AN-CFs should be a promising electrode material for CDI application.
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