期刊
JOURNAL OF ALLOYS AND COMPOUNDS
卷 721, 期 -, 页码 622-627出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.jallcom.2017.06.030
关键词
AgI; BiVO4; Photocatalysis; Degradation; Antibacterial; Visible light
资金
- National Natural Science Foundation of China [51131008, 41476068]
- National Key Basic Research Program of China [2014CB643304]
- Key Research and Development Program of Shandong Province [2015GSF115031]
- Science & Technology Basic Research Program of Qingdao [15-9-1-31-jch]
Novel Agl/BiVO4 photocatalysts were successfully synthesized via a simple hydrothermal process for the first time. The synthesized Agl/BiVO4 composites were characterized by X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), Energy dispersive spectroscopy (EDS), High resolution transmission electron microscopy (HRTEM), Scanning electron microscope (SEM), photoluminescence (PL) spectra and DV diffuse reflectance spectroscopy (UV-DRS) techniques, respectively. The photocatalytic performances of the as-obtained samples were evaluated by photodegradation of rhodamine B (RhB) and killing of Pseudomonas aeruginosa (P. aeruginosa) under visible light irradiation. The 20% Agl/BiVO4 showed higher photodegradation and photocatalytic antibacterial activity than the pure AgI and BiVO4. 20% Agl/BiVO4 exhibits the best photocatalytic performance with almost all RhB decomposed within 150 min and the antibacterial rate could achieve over 99.99% after 30 min photocatalytic antibacterial reaction. The photocatalytic antibacterial mechanism of AgliBiVO(4) was investigated by radical trapping experiments. The results revealed that superoxide radical (center dot O (2) over bar) and holes (h(+)) were the dominant active species in the photocatalytic antibacterial process. Furthermore, the 20% AgI/BiVO4 still maintained a high activity after five cycle for killing of P. aeruginosa. The experimental results showed that the synthesized AgliBiVO(4) can be used in water treatment of degradating the organic pollutants and killing the water bacteria at the same time. (C) 2017 Elsevier B.V. All rights reserved.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据