期刊
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
卷 2017, 期 18, 页码 2561-2567出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201700201
关键词
Donor-acceptor cyclopropanes; Nitriles; Cycloaddition; Lewis acids; Nitrogen heterocycles; Natural products
资金
- University of Western Ontario
- Natural Sciences and Engineering Research Council of Canada
Lewis acid promoted cycloaddition reactions of donor-acceptor (DA) cyclopropanes are one of the well-studied approaches for the construction of heterocyclic and carbocyclic frameworks. During our efforts to exploit this strategy for the synthesis and functionalization of carbohydrate-derived systems, we discovered the cycloaddition of nitriles with DA cyclopropanes. This personal account details our contributions to the development of this cycloaddition. The reaction discovery, methods development, and application in total synthesis along with related examples from others are discussed herein.
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