期刊
ORGANIC LETTERS
卷 18, 期 3, 页码 392-395出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b03399
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资金
- NSFC [21402200]
- The 100 Talents Program (The Chinese Academy of Sciences)
Copper catalyzed 1,2-alkylesterification of 1,3-dienes with diacyl peroxides affords branched allylic esters in excellent regioselectivity, including products with a newly generated fully substituted carbon center. The only byproduct is CO2. The reaction proceeds by a radical mechanism as suggested by spin trap and crossover experiments.
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