期刊
ORGANIC LETTERS
卷 18, 期 6, 页码 1494-1496出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b00338
关键词
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资金
- JSPS KAKENHI [25221301, 26713001]
- Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT)
- Japan Agency for Medical Research and Development (AMED)
- Grants-in-Aid for Scientific Research [26713001] Funding Source: KAKEN
The total synthesis of lycopalhine A has been accomplished. The synthesis features construction of the tricyclic system via cleavage of a cyclopropane ring and an ensuing intramolecular Michael addition, stereoselective introduction of a 2-aminoethyl moiety via a reaction of allyltrimethylsilane to a sulfonyliminium ion, and a stereo selective intramolecular aldol reaction.
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